FACTORS AFFECTING METHYL-CHLORIDE EMISSIONS FROM FOREST BIOMASS COMBUSTION

被引:29
作者
REINHARDT, TE [1 ]
WARD, DE [1 ]
机构
[1] US FOREST SERV,PACIFIC NW RES STN,SEATTLE,WA 98105
关键词
D O I
10.1021/es00003a034
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Chloromethane (CH3Cl or methyl chloride) is a trace gas in the atmosphere that is a characteristic emission of vegetative biomass burning. Measurements of chloromethane emissions from laboratory-scale fires in forest fuels show that CH3Cl emission factors vary considerably between flaming and smoldering combustion. Regression analysis indicates that CH3Cl emission factors can be predicted from three fire and fuel parameters: combustion efficiency, rate of heat release, and fuel chloride content. The percentage of chlorine in the fine particle emissions from burning forest fuels also varies with combustion conditions. A combustion reaction mechanism is proposed to explain the observed variation in chlorinated emissions.
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页码:825 / 832
页数:8
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