AN OPINION ON THE HETEROGENEOUS PHOTOREACTIONS OF N-2 WITH H2O

被引:41
作者
EDWARDS, JG
DAVIES, JA
BOUCHER, DL
MENNAD, A
机构
[1] Department of Chemistry, University of Toledo, Toledo, Ohio
来源
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION IN ENGLISH | 1992年 / 31卷 / 04期
关键词
D O I
10.1002/anie.199204801
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The artificial photosynthesis of ammonia, that is, the fixation of N2 and conversion to NH3, is a fascinating research goal about which there are repeated reports of success in the literature. This communication now shows amongst other results why the obvious methods, in particular the heterogeneous catalysis of the reaction of N2 and H2O on the surface of oxidic compounds, are destined to failure.
引用
收藏
页码:480 / 482
页数:3
相关论文
共 27 条
  • [1] AUGUSTYNSKI J, 1988, STRUCT BOND, V69, P20
  • [2] BOUCHER DL, 1992, THESIS U TOLEDO
  • [3] ENDOH E, 1987, NEW J CHEM, V11, P217
  • [4] HETEROGENEOUS PHOTOREDUCTION OF NITROGEN TO AMMONIA ON TUNGSTEN-OXIDE
    ENDOH, E
    LELAND, JK
    BARD, AJ
    [J]. JOURNAL OF PHYSICAL CHEMISTRY, 1986, 90 (23) : 6223 - 6226
  • [5] GOPALARAO G, 1939, Z PHYS CHEM A LPZ, V184, P377
  • [6] GOPALARAO G, 1941, J INDIAN CHEM SOC, V12, P127
  • [7] GOPOLARAO G, 1941, J INDIAN CHEM SOC, V18, P361
  • [8] PHOTOASSISTED CATALYTIC DISSOCIATION OF H2O AND REDUCTION OF N-2 TO NH3 ON PARTIALLY REDUCED FE2O3
    KHADER, MM
    LICHTIN, NN
    VURENS, GH
    SALMERON, M
    SOMORJAI, GA
    [J]. LANGMUIR, 1987, 3 (02) : 303 - 304
  • [9] KUNGSAWASD M, 1990, THESIS U TOLEDO
  • [10] AMMONIA IN HUMAN AIRWAYS - NEUTRALIZATION OF INSPIRED ACID SULFATE AEROSOLS
    LARSON, TV
    COVERT, DS
    FRANK, R
    CHARLSON, RJ
    [J]. SCIENCE, 1977, 197 (4299) : 161 - 163