DUAL-BEAM SUBPICOSECOND BROAD-BAND INFRARED SPECTROMETER

被引:59
作者
DOUGHERTY, TP
HEILWEIL, EJ
机构
[1] Molecular Physics Division, National Institute of Standards and Technology, Gaithersburg, MD, 20899
关键词
D O I
10.1364/OL.19.000129
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
A method for obtaining broadband multichannel IR spectra with subpicosecond time resolution is described. Spectrally broad IR pulses, produced by difference-frequency mixing of two visible pulses in LiIO3, are split to make signal and reference pulses. After sample absorption, the IR pulses are upconverted by a second LiIO3 crystal to produce visible pulses that are dispersed on a CCD detector to yield transient spectra with 100-cm(-1) bandwidth and 4-cm(-1) resolution. With this dual-beam technique, spectra with sensitivities of 0.001 Delta OD are obtained.
引用
收藏
页码:129 / 131
页数:3
相关论文
共 6 条
[1]   FEMTOSECOND INFRARED-SPECTROSCOPY - ULTRAFAST PHOTOCHEMISTRY OF IRON CARBONYLS IN SOLUTION [J].
ANFINRUD, PA ;
HAN, CH ;
LIAN, TQ ;
HOCHSTRASSER, RM .
JOURNAL OF PHYSICAL CHEMISTRY, 1991, 95 (02) :574-578
[2]   STRUCTURES AND KINETICS OF CR(CO)5 AND CR(CO)5.H2O IN CYCLOHEXANE SOLUTION - FLASH-PHOTOLYSIS STUDY OF CR(CO)6 WITH INFRARED AND VISIBLE DETECTION [J].
CHURCH, SP ;
GREVELS, FW ;
HERMANN, H ;
SCHAFFNER, K .
INORGANIC CHEMISTRY, 1985, 24 (03) :418-422
[3]  
GLOWNIA JUH, 1991, PHOTONICS NONLINEAR, P137
[4]   PICOSECOND TRANSIENT SPECTROSCOPY OF MOLECULES IN SOLUTION [J].
GREENE, BI ;
HOCHSTRASSER, RM ;
WEISMAN, RB .
JOURNAL OF CHEMICAL PHYSICS, 1979, 70 (03) :1247-1259
[6]   PICOSECOND TIME-RESOLVED VIBRATIONAL SPECTROSCOPY USING A REGENERATIVE AMPLIFIER [J].
JEDJU, TM ;
ROBERSON, MW ;
ROTHBERG, L .
APPLIED OPTICS, 1992, 31 (15) :2684-2691