CROSS-MEMBRANE COUPLING OF CHEMICAL SPATIOTEMPORAL PATTERNS

被引:97
作者
WINSTON, D [1 ]
ARORA, M [1 ]
MASELKO, J [1 ]
GASPAR, V [1 ]
SHOWALTER, K [1 ]
机构
[1] W VIRGINIA UNIV,DEPT CHEM,MORGANTOWN,WV 26506
关键词
D O I
10.1038/351132a0
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
CHEMICAL systems may communicate by exchange of common species through mass transport, and such coupling may give rise to dynamical complexity beyond that possible in the independent systems 1-5. We report here on dynamical behaviour arising from the diffusive coupling of chemical spatiotemporal patterns across a membrane. Chemical waves appear on Nafion membranes that are loaded with ferroin catalyst and bathed in a mixture of the reagents of the Belousv-Zhabotinsky oscillatory reaction. The waves on each side of the membrane couple by diffusive transport through the membrane. The coupling initially gives rise to the spontaneous appearance of spiral waves, and subsequent behaviour reveals several distinct phases of evolution, ultimately leading to complete spatiotemporal entrainment.
引用
收藏
页码:132 / 135
页数:4
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