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ROTATIONALLY RESOLVED ULTRAVIOLET-SPECTRUM OF THE BENZENE-AR COMPLEX BY MASS-SELECTED RESONANCE-ENHANCED 2-PHOTON IONIZATION
被引:183
作者
:
WEBER, T
论文数:
0
引用数:
0
h-index:
0
机构:
Institut für Physikalische und Theoretische Chemie, Technische Universität München, D-8046 Garching
WEBER, T
VONBARGEN, A
论文数:
0
引用数:
0
h-index:
0
机构:
Institut für Physikalische und Theoretische Chemie, Technische Universität München, D-8046 Garching
VONBARGEN, A
RIEDLE, E
论文数:
0
引用数:
0
h-index:
0
机构:
Institut für Physikalische und Theoretische Chemie, Technische Universität München, D-8046 Garching
RIEDLE, E
NEUSSER, HJ
论文数:
0
引用数:
0
h-index:
0
机构:
Institut für Physikalische und Theoretische Chemie, Technische Universität München, D-8046 Garching
NEUSSER, HJ
机构
:
[1]
Institut für Physikalische und Theoretische Chemie, Technische Universität München, D-8046 Garching
来源
:
JOURNAL OF CHEMICAL PHYSICS
|
1990年
/ 92卷
/ 01期
关键词
:
D O I
:
10.1063/1.458394
中图分类号
:
O64 [物理化学(理论化学)、化学物理学];
学科分类号
:
070304 ;
081704 ;
摘要
:
High resolution laser excitation was combined with the technique of mass-selected two-photon ionization via a resonant intermediate state to measure rotationally resolved UV spectra of benzene-Ar van der Waals clusters. When the second laser pulse in the two color experiment is delayed by 7 ns no line broadening due to the second ionizing absorption step is observed. Spectra of three vibronic bands in the S1 ← S0 transition of benzene (h6)-Ar and benzene (d6)-Ar were measured yielding a line spectrum with a linewidth of 130 MHz. Resolution is sufficient to demonstrate that no asymmetry splitting of the rotational lines occurs and the spectrum is to a high precision that of a symmetric rotor. A detailed analysis of the rotational structure yields an accurate set of rotational constants. We find that the Ar is located on the C6 rotational axis. Its distance from the benzene ring plane is 3.582 Å in the electronic ground state and decreases by 59 ± 3 mÅ in the electronically excited state due to the increased polarizability of the benzene molecule after electronic excitation. © 1990 American Institute of Physics.
引用
收藏
页码:90 / 96
页数:7
相关论文
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[1]
BALOCCHI FA, 1983, J PHYS CHEM-US, V87, P2079, DOI 10.1021/j100235a012
[2]
ROTATIONAL ANALYSIS OF THE 1B2U(PI-PI-STAR) ]-1A1G(610) BAND OF BENZENE AND HELIUM-BENZENE VANDERWAALS COMPLEXES IN A SUPERSONIC JET
[J].
BECK, SM
论文数:
0
引用数:
0
h-index:
0
机构:
Department of Chemistry, William Marsh Rice University, Houston
BECK, SM
;
LIVERMAN, MG
论文数:
0
引用数:
0
h-index:
0
机构:
Department of Chemistry, William Marsh Rice University, Houston
LIVERMAN, MG
;
MONTS, DL
论文数:
0
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0
h-index:
0
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Department of Chemistry, William Marsh Rice University, Houston
MONTS, DL
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SMALLEY, RE
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引用数:
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Department of Chemistry, William Marsh Rice University, Houston
SMALLEY, RE
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JOURNAL OF CHEMICAL PHYSICS,
1979,
70
(01)
:232
-237
[3]
IONIZATION-POTENTIALS OF LARGE VANDERWAALS MOLECULES
[J].
BENHORIN, N
论文数:
0
引用数:
0
h-index:
0
BENHORIN, N
;
EVEN, U
论文数:
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引用数:
0
h-index:
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EVEN, U
;
JORTNER, J
论文数:
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引用数:
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h-index:
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JORTNER, J
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JOURNAL OF CHEMICAL PHYSICS,
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[4]
ISOTOPE SELECTIVE SOFT MULTI-PHOTON IONIZATION AND FRAGMENTATION OF POLYATOMIC-MOLECULES
[J].
BOESL, U
论文数:
0
引用数:
0
h-index:
0
机构:
TECH UNIV MUNICH,INST PHYS & THEORET CHEM,D-8046 GARCHING,FED REP GER
TECH UNIV MUNICH,INST PHYS & THEORET CHEM,D-8046 GARCHING,FED REP GER
BOESL, U
;
NEUSSER, HJ
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0
引用数:
0
h-index:
0
机构:
TECH UNIV MUNICH,INST PHYS & THEORET CHEM,D-8046 GARCHING,FED REP GER
TECH UNIV MUNICH,INST PHYS & THEORET CHEM,D-8046 GARCHING,FED REP GER
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TECH UNIV MUNICH,INST PHYS & THEORET CHEM,D-8046 GARCHING,FED REP GER
SCHLAG, EW
.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,
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NEW S1-VIBRONIC LEVEL ASSIGNMENTS FOR S-TETRAZINE VAPOR - POLARIZATION AND LIFETIME MEASUREMENTS
[J].
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0
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UNIV CHICAGO, JAMES FRANCK INST, CHICAGO, IL 60637 USA
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HAYNAM, CA
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HAYNAM, CA
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JOURNAL OF MOLECULAR SPECTROSCOPY,
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CLUSTERS - PROPERTIES AND FORMATION
[J].
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ANNUAL REVIEW OF PHYSICAL CHEMISTRY,
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37
:525
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[7]
DETERMINATION OF THE IONIZATION-ENERGY OF THE BENZENE ARGON COMPLEX BY ZERO KINETIC-ENERGY PHOTOELECTRON-SPECTROSCOPY
[J].
CHEWTER, LA
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0
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TECH UNIV MUNICH,INST PHYS & THEORET CHEM,LICHTENBERGSTR 4,D-8046 GARCHING,FED REP GER
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SUB-DOPPLER LASER SPECTROSCOPY OF NO2 IN THE LAMBDA = 592.5-NM REGION
[J].
FOTH, HJ
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FOTH, HJ
;
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[J].
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TECH UNIV MUNICH,INST PHYS & THEORET CHEM,D-8046 GARCHING,FED REP GER
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IONIZATION-POTENTIAL OF THE BENZENE-ARGON COMPLEX IN A JET
[J].
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TECH UNIV MUNICH,D-8046 GARCHING,FED REP GER
TECH UNIV MUNICH,D-8046 GARCHING,FED REP GER
FUNG, KH
;
HENKE, WE
论文数:
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h-index:
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TECH UNIV MUNICH,D-8046 GARCHING,FED REP GER
HENKE, WE
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论文数:
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引用数:
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TECH UNIV MUNICH,D-8046 GARCHING,FED REP GER
TECH UNIV MUNICH,D-8046 GARCHING,FED REP GER
HAYS, TR
;
SELZLE, HL
论文数:
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引用数:
0
h-index:
0
机构:
TECH UNIV MUNICH,D-8046 GARCHING,FED REP GER
TECH UNIV MUNICH,D-8046 GARCHING,FED REP GER
SELZLE, HL
;
SCHLAG, EW
论文数:
0
引用数:
0
h-index:
0
机构:
TECH UNIV MUNICH,D-8046 GARCHING,FED REP GER
TECH UNIV MUNICH,D-8046 GARCHING,FED REP GER
SCHLAG, EW
.
JOURNAL OF PHYSICAL CHEMISTRY,
1981,
85
(24)
:3560
-3563
←
1
2
3
4
→
共 33 条
[1]
BALOCCHI FA, 1983, J PHYS CHEM-US, V87, P2079, DOI 10.1021/j100235a012
[2]
ROTATIONAL ANALYSIS OF THE 1B2U(PI-PI-STAR) ]-1A1G(610) BAND OF BENZENE AND HELIUM-BENZENE VANDERWAALS COMPLEXES IN A SUPERSONIC JET
[J].
BECK, SM
论文数:
0
引用数:
0
h-index:
0
机构:
Department of Chemistry, William Marsh Rice University, Houston
BECK, SM
;
LIVERMAN, MG
论文数:
0
引用数:
0
h-index:
0
机构:
Department of Chemistry, William Marsh Rice University, Houston
LIVERMAN, MG
;
MONTS, DL
论文数:
0
引用数:
0
h-index:
0
机构:
Department of Chemistry, William Marsh Rice University, Houston
MONTS, DL
;
SMALLEY, RE
论文数:
0
引用数:
0
h-index:
0
机构:
Department of Chemistry, William Marsh Rice University, Houston
SMALLEY, RE
.
JOURNAL OF CHEMICAL PHYSICS,
1979,
70
(01)
:232
-237
[3]
IONIZATION-POTENTIALS OF LARGE VANDERWAALS MOLECULES
[J].
BENHORIN, N
论文数:
0
引用数:
0
h-index:
0
BENHORIN, N
;
EVEN, U
论文数:
0
引用数:
0
h-index:
0
EVEN, U
;
JORTNER, J
论文数:
0
引用数:
0
h-index:
0
JORTNER, J
.
JOURNAL OF CHEMICAL PHYSICS,
1989,
91
(01)
:331
-339
[4]
ISOTOPE SELECTIVE SOFT MULTI-PHOTON IONIZATION AND FRAGMENTATION OF POLYATOMIC-MOLECULES
[J].
BOESL, U
论文数:
0
引用数:
0
h-index:
0
机构:
TECH UNIV MUNICH,INST PHYS & THEORET CHEM,D-8046 GARCHING,FED REP GER
TECH UNIV MUNICH,INST PHYS & THEORET CHEM,D-8046 GARCHING,FED REP GER
BOESL, U
;
NEUSSER, HJ
论文数:
0
引用数:
0
h-index:
0
机构:
TECH UNIV MUNICH,INST PHYS & THEORET CHEM,D-8046 GARCHING,FED REP GER
TECH UNIV MUNICH,INST PHYS & THEORET CHEM,D-8046 GARCHING,FED REP GER
NEUSSER, HJ
;
SCHLAG, EW
论文数:
0
引用数:
0
h-index:
0
机构:
TECH UNIV MUNICH,INST PHYS & THEORET CHEM,D-8046 GARCHING,FED REP GER
TECH UNIV MUNICH,INST PHYS & THEORET CHEM,D-8046 GARCHING,FED REP GER
SCHLAG, EW
.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,
1981,
103
(17)
:5058
-5060
[5]
NEW S1-VIBRONIC LEVEL ASSIGNMENTS FOR S-TETRAZINE VAPOR - POLARIZATION AND LIFETIME MEASUREMENTS
[J].
BRUMBAUGH, DV
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV CHICAGO, JAMES FRANCK INST, CHICAGO, IL 60637 USA
BRUMBAUGH, DV
;
HAYNAM, CA
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV CHICAGO, JAMES FRANCK INST, CHICAGO, IL 60637 USA
HAYNAM, CA
;
LEVY, DH
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV CHICAGO, JAMES FRANCK INST, CHICAGO, IL 60637 USA
LEVY, DH
.
JOURNAL OF MOLECULAR SPECTROSCOPY,
1982,
94
(02)
:316
-335
[6]
CLUSTERS - PROPERTIES AND FORMATION
[J].
CASTLEMAN, AW
论文数:
0
引用数:
0
h-index:
0
CASTLEMAN, AW
;
KEESEE, RG
论文数:
0
引用数:
0
h-index:
0
KEESEE, RG
.
ANNUAL REVIEW OF PHYSICAL CHEMISTRY,
1986,
37
:525
-550
[7]
DETERMINATION OF THE IONIZATION-ENERGY OF THE BENZENE ARGON COMPLEX BY ZERO KINETIC-ENERGY PHOTOELECTRON-SPECTROSCOPY
[J].
CHEWTER, LA
论文数:
0
引用数:
0
h-index:
0
机构:
TECH UNIV MUNICH,INST PHYS & THEORET CHEM,LICHTENBERGSTR 4,D-8046 GARCHING,FED REP GER
TECH UNIV MUNICH,INST PHYS & THEORET CHEM,LICHTENBERGSTR 4,D-8046 GARCHING,FED REP GER
CHEWTER, LA
;
MULLERDETHLEFS, K
论文数:
0
引用数:
0
h-index:
0
机构:
TECH UNIV MUNICH,INST PHYS & THEORET CHEM,LICHTENBERGSTR 4,D-8046 GARCHING,FED REP GER
TECH UNIV MUNICH,INST PHYS & THEORET CHEM,LICHTENBERGSTR 4,D-8046 GARCHING,FED REP GER
MULLERDETHLEFS, K
;
SCHLAG, EW
论文数:
0
引用数:
0
h-index:
0
机构:
TECH UNIV MUNICH,INST PHYS & THEORET CHEM,LICHTENBERGSTR 4,D-8046 GARCHING,FED REP GER
TECH UNIV MUNICH,INST PHYS & THEORET CHEM,LICHTENBERGSTR 4,D-8046 GARCHING,FED REP GER
SCHLAG, EW
.
CHEMICAL PHYSICS LETTERS,
1987,
135
(03)
:219
-222
[8]
SUB-DOPPLER LASER SPECTROSCOPY OF NO2 IN THE LAMBDA = 592.5-NM REGION
[J].
FOTH, HJ
论文数:
0
引用数:
0
h-index:
0
FOTH, HJ
;
VEDDER, HJ
论文数:
0
引用数:
0
h-index:
0
VEDDER, HJ
;
DEMTRODER, W
论文数:
0
引用数:
0
h-index:
0
DEMTRODER, W
.
JOURNAL OF MOLECULAR SPECTROSCOPY,
1981,
88
(01)
:109
-125
[9]
STUDY OF ISOTOPE EFFECTS IN BENZENE DIMERS IN A SEEDED SUPERSONIC JET
[J].
FUNG, KH
论文数:
0
引用数:
0
h-index:
0
机构:
TECH UNIV MUNICH,INST PHYS & THEORET CHEM,D-8046 GARCHING,FED REP GER
TECH UNIV MUNICH,INST PHYS & THEORET CHEM,D-8046 GARCHING,FED REP GER
FUNG, KH
;
SELZLE, HL
论文数:
0
引用数:
0
h-index:
0
机构:
TECH UNIV MUNICH,INST PHYS & THEORET CHEM,D-8046 GARCHING,FED REP GER
TECH UNIV MUNICH,INST PHYS & THEORET CHEM,D-8046 GARCHING,FED REP GER
SELZLE, HL
;
SCHLAG, EW
论文数:
0
引用数:
0
h-index:
0
机构:
TECH UNIV MUNICH,INST PHYS & THEORET CHEM,D-8046 GARCHING,FED REP GER
TECH UNIV MUNICH,INST PHYS & THEORET CHEM,D-8046 GARCHING,FED REP GER
SCHLAG, EW
.
JOURNAL OF PHYSICAL CHEMISTRY,
1983,
87
(25)
:5113
-5116
[10]
IONIZATION-POTENTIAL OF THE BENZENE-ARGON COMPLEX IN A JET
[J].
FUNG, KH
论文数:
0
引用数:
0
h-index:
0
机构:
TECH UNIV MUNICH,D-8046 GARCHING,FED REP GER
TECH UNIV MUNICH,D-8046 GARCHING,FED REP GER
FUNG, KH
;
HENKE, WE
论文数:
0
引用数:
0
h-index:
0
机构:
TECH UNIV MUNICH,D-8046 GARCHING,FED REP GER
TECH UNIV MUNICH,D-8046 GARCHING,FED REP GER
HENKE, WE
;
HAYS, TR
论文数:
0
引用数:
0
h-index:
0
机构:
TECH UNIV MUNICH,D-8046 GARCHING,FED REP GER
TECH UNIV MUNICH,D-8046 GARCHING,FED REP GER
HAYS, TR
;
SELZLE, HL
论文数:
0
引用数:
0
h-index:
0
机构:
TECH UNIV MUNICH,D-8046 GARCHING,FED REP GER
TECH UNIV MUNICH,D-8046 GARCHING,FED REP GER
SELZLE, HL
;
SCHLAG, EW
论文数:
0
引用数:
0
h-index:
0
机构:
TECH UNIV MUNICH,D-8046 GARCHING,FED REP GER
TECH UNIV MUNICH,D-8046 GARCHING,FED REP GER
SCHLAG, EW
.
JOURNAL OF PHYSICAL CHEMISTRY,
1981,
85
(24)
:3560
-3563
←
1
2
3
4
→