QUANTUM SIZED SEMICONDUCTOR PARTICLES IN SOLUTION AND IN MODIFIED LAYERS

被引:64
作者
WELLER, H
机构
来源
BERICHTE DER BUNSEN-GESELLSCHAFT-PHYSICAL CHEMISTRY CHEMICAL PHYSICS | 1991年 / 95卷 / 11期
关键词
COLLOIDS; MATERIALS PROPERTIES; PHOTOCHEMISTRY; PHOTOELECTROCHEMISTRY;
D O I
10.1002/bbpc.19910951108
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The preparation of highly monodisperse, quantum-sized CdS particles is described. In these samples a band splitting into discrete exciton-like states is observed. - Quantum-sized CdS and PbS particles prepared in situ on highly porous, polycrystalline TiO2 electrodes work as highly efficient sensitizers. Photocurrent yields of more than 70% are reported. In the case of PbS it is shown that an efficient electron transfer is only possible with particles in the size quantization regime.
引用
收藏
页码:1361 / 1365
页数:5
相关论文
共 14 条
[1]   ZERO-DIMENSIONAL EXCITONS IN SEMICONDUCTOR CLUSTERS [J].
BRUS, L .
IEEE JOURNAL OF QUANTUM ELECTRONICS, 1986, 22 (09) :1909-1914
[2]  
CUFF KF, 1964, 7 P INT C PHYS SEM, P677
[3]   PHOTOCHEMISTRY OF SEMICONDUCTOR COLLOIDS .35. SIZE SEPARATION OF COLLOIDAL CDS BY GEL-ELECTROPHORESIS [J].
EYCHMULLER, A ;
KATSIKAS, L ;
WELLER, H .
LANGMUIR, 1990, 6 (10) :1605-1608
[4]   PHOTOCHEMISTRY OF COLLOIDAL SEMICONDUCTORS .30. HPLC INVESTIGATION OF SMALL CDS PARTICLES [J].
FISCHER, CH ;
WELLER, H ;
KATSIKAS, L ;
HENGLEIN, A .
LANGMUIR, 1989, 5 (02) :429-432
[5]   PHOTOCHEMISTRY OF COLLOIDAL SEMICONDUCTORS .29. FRACTIONATION OF CDS SOLS OF SMALL PARTICLES BY EXCLUSION CHROMATOGRAPHY [J].
FISCHER, CH ;
LILIE, J ;
WELLER, H ;
KATSIKAS, L ;
HENGLEIN, A .
BERICHTE DER BUNSEN-GESELLSCHAFT-PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 1989, 93 (01) :61-64
[6]  
HAASE M, IN PRESS
[7]  
HENGLEIN A, 1988, TOP CURR CHEM, V143, P113
[9]   DISCRETE EXCITONIC TRANSITIONS IN QUANTUM-SIZED CDS PARTICLES [J].
KATSIKAS, L ;
EYCHMULLER, A ;
GIERSIG, M ;
WELLER, H .
CHEMICAL PHYSICS LETTERS, 1990, 172 (3-4) :201-204
[10]   PHOTOCHEMISTRY OF COLLOIDAL SEMICONDUCTORS .15. QUANTUM SIZE EFFECTS IN SEMICONDUCTOR CRYSTALLITES - CALCULATION OF THE ENERGY-SPECTRUM FOR THE CONFINED EXCITON [J].
SCHMIDT, HM ;
WELLER, H .
CHEMICAL PHYSICS LETTERS, 1986, 129 (06) :615-618