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PHOTOELECTRON-SPECTROSCOPY OF TRANSITION-METAL CLUSTERS - CORRELATION OF VALENCE ELECTRONIC-STRUCTURE TO REACTIVITY
被引:81
作者
:
CONCEICAO, J
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
CONCEICAO, J
LAAKSONEN, RT
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
LAAKSONEN, RT
WANG, LS
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
WANG, LS
GUO, T
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
GUO, T
NORDLANDER, P
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
NORDLANDER, P
SMALLEY, RE
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
SMALLEY, RE
机构
:
[1]
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
[2]
RICE UNIV,RICE QUANTUM INST,HOUSTON,TX 77251
来源
:
PHYSICAL REVIEW B
|
1995年
/ 51卷
/ 07期
关键词
:
D O I
:
10.1103/PhysRevB.51.4668
中图分类号
:
T [工业技术];
学科分类号
:
08 ;
摘要
:
The photoelectron spectra and the reactivity of H2 with Fe, Co, and Ni clusters have been studied as a function of cluster size for clusters ranging from 5 to 26 atoms in size. It is shown that the variation of the reactivity correlates with the variation of the difference between the ionization potential and the electron affinity of the clusters. This finding is rationalized by using a simple model in which the probability of H2 chemisorption on the cluster is proportional to the magnitude of an entrance channel barrier caused by Pauli repulsion between H2 and the cluster. It is argued that the magnitude of this barrier is proportional to the promotion energy of an electron from the frontier orbital of the cluster to the lowest unoccupied d state of the cluster. © 1995 The American Physical Society.
引用
收藏
页码:4668 / 4671
页数:4
相关论文
共 26 条
[1]
CHEMISTRY OF EXCITED ELECTRONIC STATES
ARMENTROUT, PB
论文数:
0
引用数:
0
h-index:
0
机构:
Department of Chemistry, University of Utah, Salt Lake City
ARMENTROUT, PB
[J].
SCIENCE,
1991,
251
(4990)
: 175
-
179
[2]
MAGNETIC TIME-OF-FLIGHT PHOTOELECTRON SPECTROMETER FOR MASS-SELECTED NEGATIVE CLUSTER IONS
CHESHNOVSKY, O
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
CHESHNOVSKY, O
YANG, SH
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
YANG, SH
PETTIETTE, CL
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
PETTIETTE, CL
CRAYCRAFT, MJ
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
CRAYCRAFT, MJ
SMALLEY, RE
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
SMALLEY, RE
[J].
REVIEW OF SCIENTIFIC INSTRUMENTS,
1987,
58
(11)
: 2131
-
2137
[3]
LASER PHOTOELECTRON SPECTROMETRY OF CO- AND NI-
CORDERMAN, RR
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV COLORADO,JOINT INST LAB ASTROPHYS,BOULDER,CO 80309
CORDERMAN, RR
ENGELKING, PC
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV COLORADO,JOINT INST LAB ASTROPHYS,BOULDER,CO 80309
ENGELKING, PC
LINEBERGER, WC
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV COLORADO,JOINT INST LAB ASTROPHYS,BOULDER,CO 80309
LINEBERGER, WC
[J].
JOURNAL OF CHEMICAL PHYSICS,
1979,
70
(10)
: 4474
-
4480
[4]
FOURIER-TRANSFORM ION-CYCLOTRON RESONANCE STUDIES OF H-2 CHEMISORPTION ON NIOBIUM CLUSTER CATIONS
ELKIND, JL
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
ELKIND, JL
WEISS, FD
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
WEISS, FD
ALFORD, JM
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
ALFORD, JM
LAAKSONEN, RT
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
LAAKSONEN, RT
SMALLEY, RE
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
SMALLEY, RE
[J].
JOURNAL OF CHEMICAL PHYSICS,
1988,
88
(08)
: 5215
-
5224
[5]
PALLADIUM CLUSTERS - H-2, D-2, N-2, CH4, CD4, C2H4, AND C2H6 REACTIVITY AND D-2 SATURATION STUDIES
FAYET, P
论文数:
0
引用数:
0
h-index:
0
机构:
Corporate Research Laboratories, Exxon Research and Engineering Company, Annandale
FAYET, P
KALDOR, A
论文数:
0
引用数:
0
h-index:
0
机构:
Corporate Research Laboratories, Exxon Research and Engineering Company, Annandale
KALDOR, A
COX, DM
论文数:
0
引用数:
0
h-index:
0
机构:
Corporate Research Laboratories, Exxon Research and Engineering Company, Annandale
COX, DM
[J].
JOURNAL OF CHEMICAL PHYSICS,
1990,
92
(01)
: 254
-
261
[6]
HYDROGEN CHEMISORPTION ON TRANSITION-METAL CLUSTERS
GEUSIC, ME
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
GEUSIC, ME
MORSE, MD
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
MORSE, MD
SMALLEY, RE
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
SMALLEY, RE
[J].
JOURNAL OF CHEMICAL PHYSICS,
1985,
82
(01)
: 590
-
591
[7]
MAGIC NUMBERS FOR METALLIC CLUSTERS AND THE PRINCIPLE OF MAXIMUM HARDNESS
HARBOLA, MK
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV N CAROLINA, DEPT CHEM, CHAPEL HILL, NC 27599 USA
UNIV N CAROLINA, DEPT CHEM, CHAPEL HILL, NC 27599 USA
HARBOLA, MK
[J].
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA,
1992,
89
(03)
: 1036
-
1039
[8]
THE INTERACTION OF H-2 WITH METAL-SURFACES
HARRIS, J
论文数:
0
引用数:
0
h-index:
0
机构:
CHALMERS UNIV TECHNOL, S-41296 GOTHENBURG, SWEDEN
CHALMERS UNIV TECHNOL, S-41296 GOTHENBURG, SWEDEN
HARRIS, J
ANDERSSON, S
论文数:
0
引用数:
0
h-index:
0
机构:
CHALMERS UNIV TECHNOL, S-41296 GOTHENBURG, SWEDEN
CHALMERS UNIV TECHNOL, S-41296 GOTHENBURG, SWEDEN
ANDERSSON, S
HOLMBERG, C
论文数:
0
引用数:
0
h-index:
0
机构:
CHALMERS UNIV TECHNOL, S-41296 GOTHENBURG, SWEDEN
CHALMERS UNIV TECHNOL, S-41296 GOTHENBURG, SWEDEN
HOLMBERG, C
NORDLANDER, P
论文数:
0
引用数:
0
h-index:
0
机构:
CHALMERS UNIV TECHNOL, S-41296 GOTHENBURG, SWEDEN
CHALMERS UNIV TECHNOL, S-41296 GOTHENBURG, SWEDEN
NORDLANDER, P
[J].
PHYSICA SCRIPTA,
1986,
T13
: 155
-
160
[9]
H-2 DISSOCIATION AT METAL-SURFACES
HARRIS, J
论文数:
0
引用数:
0
h-index:
0
机构:
CHALMERS UNIV TECHNOL, DEPT PHYS, S-41296 GOTHENBURG, SWEDEN
CHALMERS UNIV TECHNOL, DEPT PHYS, S-41296 GOTHENBURG, SWEDEN
HARRIS, J
ANDERSSON, S
论文数:
0
引用数:
0
h-index:
0
机构:
CHALMERS UNIV TECHNOL, DEPT PHYS, S-41296 GOTHENBURG, SWEDEN
CHALMERS UNIV TECHNOL, DEPT PHYS, S-41296 GOTHENBURG, SWEDEN
ANDERSSON, S
[J].
PHYSICAL REVIEW LETTERS,
1985,
55
(15)
: 1583
-
1586
[10]
PHOTOELECTRON-SPECTROSCOPY OF METAL CLUSTER ANIONS - CUN-, AGN-, AND AUN-
HO, J
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV COLORADO,NIST,JOINT INST LAB ASTROPHYS,BOULDER,CO 80309
UNIV COLORADO,NIST,JOINT INST LAB ASTROPHYS,BOULDER,CO 80309
HO, J
ERVIN, KM
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV COLORADO,NIST,JOINT INST LAB ASTROPHYS,BOULDER,CO 80309
UNIV COLORADO,NIST,JOINT INST LAB ASTROPHYS,BOULDER,CO 80309
ERVIN, KM
LINEBERGER, WC
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV COLORADO,NIST,JOINT INST LAB ASTROPHYS,BOULDER,CO 80309
UNIV COLORADO,NIST,JOINT INST LAB ASTROPHYS,BOULDER,CO 80309
LINEBERGER, WC
[J].
JOURNAL OF CHEMICAL PHYSICS,
1990,
93
(10)
: 6987
-
7002
←
1
2
3
→
共 26 条
[1]
CHEMISTRY OF EXCITED ELECTRONIC STATES
ARMENTROUT, PB
论文数:
0
引用数:
0
h-index:
0
机构:
Department of Chemistry, University of Utah, Salt Lake City
ARMENTROUT, PB
[J].
SCIENCE,
1991,
251
(4990)
: 175
-
179
[2]
MAGNETIC TIME-OF-FLIGHT PHOTOELECTRON SPECTROMETER FOR MASS-SELECTED NEGATIVE CLUSTER IONS
CHESHNOVSKY, O
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
CHESHNOVSKY, O
YANG, SH
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
YANG, SH
PETTIETTE, CL
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
PETTIETTE, CL
CRAYCRAFT, MJ
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
CRAYCRAFT, MJ
SMALLEY, RE
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
SMALLEY, RE
[J].
REVIEW OF SCIENTIFIC INSTRUMENTS,
1987,
58
(11)
: 2131
-
2137
[3]
LASER PHOTOELECTRON SPECTROMETRY OF CO- AND NI-
CORDERMAN, RR
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV COLORADO,JOINT INST LAB ASTROPHYS,BOULDER,CO 80309
CORDERMAN, RR
ENGELKING, PC
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV COLORADO,JOINT INST LAB ASTROPHYS,BOULDER,CO 80309
ENGELKING, PC
LINEBERGER, WC
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV COLORADO,JOINT INST LAB ASTROPHYS,BOULDER,CO 80309
LINEBERGER, WC
[J].
JOURNAL OF CHEMICAL PHYSICS,
1979,
70
(10)
: 4474
-
4480
[4]
FOURIER-TRANSFORM ION-CYCLOTRON RESONANCE STUDIES OF H-2 CHEMISORPTION ON NIOBIUM CLUSTER CATIONS
ELKIND, JL
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
ELKIND, JL
WEISS, FD
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
WEISS, FD
ALFORD, JM
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
ALFORD, JM
LAAKSONEN, RT
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
LAAKSONEN, RT
SMALLEY, RE
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
SMALLEY, RE
[J].
JOURNAL OF CHEMICAL PHYSICS,
1988,
88
(08)
: 5215
-
5224
[5]
PALLADIUM CLUSTERS - H-2, D-2, N-2, CH4, CD4, C2H4, AND C2H6 REACTIVITY AND D-2 SATURATION STUDIES
FAYET, P
论文数:
0
引用数:
0
h-index:
0
机构:
Corporate Research Laboratories, Exxon Research and Engineering Company, Annandale
FAYET, P
KALDOR, A
论文数:
0
引用数:
0
h-index:
0
机构:
Corporate Research Laboratories, Exxon Research and Engineering Company, Annandale
KALDOR, A
COX, DM
论文数:
0
引用数:
0
h-index:
0
机构:
Corporate Research Laboratories, Exxon Research and Engineering Company, Annandale
COX, DM
[J].
JOURNAL OF CHEMICAL PHYSICS,
1990,
92
(01)
: 254
-
261
[6]
HYDROGEN CHEMISORPTION ON TRANSITION-METAL CLUSTERS
GEUSIC, ME
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
GEUSIC, ME
MORSE, MD
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
MORSE, MD
SMALLEY, RE
论文数:
0
引用数:
0
h-index:
0
机构:
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
SMALLEY, RE
[J].
JOURNAL OF CHEMICAL PHYSICS,
1985,
82
(01)
: 590
-
591
[7]
MAGIC NUMBERS FOR METALLIC CLUSTERS AND THE PRINCIPLE OF MAXIMUM HARDNESS
HARBOLA, MK
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV N CAROLINA, DEPT CHEM, CHAPEL HILL, NC 27599 USA
UNIV N CAROLINA, DEPT CHEM, CHAPEL HILL, NC 27599 USA
HARBOLA, MK
[J].
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA,
1992,
89
(03)
: 1036
-
1039
[8]
THE INTERACTION OF H-2 WITH METAL-SURFACES
HARRIS, J
论文数:
0
引用数:
0
h-index:
0
机构:
CHALMERS UNIV TECHNOL, S-41296 GOTHENBURG, SWEDEN
CHALMERS UNIV TECHNOL, S-41296 GOTHENBURG, SWEDEN
HARRIS, J
ANDERSSON, S
论文数:
0
引用数:
0
h-index:
0
机构:
CHALMERS UNIV TECHNOL, S-41296 GOTHENBURG, SWEDEN
CHALMERS UNIV TECHNOL, S-41296 GOTHENBURG, SWEDEN
ANDERSSON, S
HOLMBERG, C
论文数:
0
引用数:
0
h-index:
0
机构:
CHALMERS UNIV TECHNOL, S-41296 GOTHENBURG, SWEDEN
CHALMERS UNIV TECHNOL, S-41296 GOTHENBURG, SWEDEN
HOLMBERG, C
NORDLANDER, P
论文数:
0
引用数:
0
h-index:
0
机构:
CHALMERS UNIV TECHNOL, S-41296 GOTHENBURG, SWEDEN
CHALMERS UNIV TECHNOL, S-41296 GOTHENBURG, SWEDEN
NORDLANDER, P
[J].
PHYSICA SCRIPTA,
1986,
T13
: 155
-
160
[9]
H-2 DISSOCIATION AT METAL-SURFACES
HARRIS, J
论文数:
0
引用数:
0
h-index:
0
机构:
CHALMERS UNIV TECHNOL, DEPT PHYS, S-41296 GOTHENBURG, SWEDEN
CHALMERS UNIV TECHNOL, DEPT PHYS, S-41296 GOTHENBURG, SWEDEN
HARRIS, J
ANDERSSON, S
论文数:
0
引用数:
0
h-index:
0
机构:
CHALMERS UNIV TECHNOL, DEPT PHYS, S-41296 GOTHENBURG, SWEDEN
CHALMERS UNIV TECHNOL, DEPT PHYS, S-41296 GOTHENBURG, SWEDEN
ANDERSSON, S
[J].
PHYSICAL REVIEW LETTERS,
1985,
55
(15)
: 1583
-
1586
[10]
PHOTOELECTRON-SPECTROSCOPY OF METAL CLUSTER ANIONS - CUN-, AGN-, AND AUN-
HO, J
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV COLORADO,NIST,JOINT INST LAB ASTROPHYS,BOULDER,CO 80309
UNIV COLORADO,NIST,JOINT INST LAB ASTROPHYS,BOULDER,CO 80309
HO, J
ERVIN, KM
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV COLORADO,NIST,JOINT INST LAB ASTROPHYS,BOULDER,CO 80309
UNIV COLORADO,NIST,JOINT INST LAB ASTROPHYS,BOULDER,CO 80309
ERVIN, KM
LINEBERGER, WC
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV COLORADO,NIST,JOINT INST LAB ASTROPHYS,BOULDER,CO 80309
UNIV COLORADO,NIST,JOINT INST LAB ASTROPHYS,BOULDER,CO 80309
LINEBERGER, WC
[J].
JOURNAL OF CHEMICAL PHYSICS,
1990,
93
(10)
: 6987
-
7002
←
1
2
3
→