3RD-HARMONIC GENERATION FROM QUANTUM-STATE PBS EMBEDDED IN LANGMUIR-BLODGETT-FILM MATRIX

被引:8
作者
MORIGUCHI, I [1 ]
HANAI, K [1 ]
TERAOKA, Y [1 ]
KAGAWA, S [1 ]
YAMADA, S [1 ]
MATSUO, T [1 ]
机构
[1] KYUSHU UNIV,FAC ENGN,DEPT CHEM SCI & TECHNOL,FUKUOKA 812,JAPAN
来源
JAPANESE JOURNAL OF APPLIED PHYSICS PART 2-LETTERS | 1995年 / 34卷 / 3A期
关键词
3RD HARMONIC GENERATION; PBS; NANOCRYSTALLITE; QUANTUM-STATE; LANGMUIR-BLODGETT FILM MATRIX;
D O I
10.1143/JJAP.34.L323
中图分类号
O59 [应用物理学];
学科分类号
摘要
PbS-bearing Langmuir-Blodgett (LB) films were synthesized by alternating the processes of sulfidation by the exposure to H2S gas and intercalation of pb(2+) ions. These processes allowed the in situ formation and growth of the nano-sized (quantum-state) PbS in the hydrophilic interlayers of the stearate LB film. The third-order nonlinear optical susceptibility, ((3)(chi)), of the quantum-state PbS embedded in the LB matrix was evaluated for the first time by third harmonic generation. The PbS/LB films showed the ((3)(chi)) values of the order of 10(-12) esu, and the in situ growth of the quatum-state PbS resulted in the enhacement of ((3)(chi)).
引用
收藏
页码:L323 / L325
页数:3
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