ELECTRONIC DISTORTION IN KEV PARTICLE BOMBARDMENT

被引:15
作者
BHATIA, R
GARRISON, BJ
机构
[1] Department of Chemistry, Pennsylvania State University, University Park
关键词
D O I
10.1063/1.466742
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The angle resolved velocity distributions of excited (F-4(7/2)) and ground state (F-4(9/2)) Rh atoms ejected from the Rh {100} surface due to keV Ar+ ion bombardment are described with; a-model that takes into account the local electronic environment. The lifetime of the;e excitation probability for each excited Rh atom is assumed to depend on the local embedded-atom method (EAM) density. It is thus possible to distinguish between ejected atoms that experience very little difference in their electronic environments, Although most excited atoms that survive with significantly high excitation probabilities originate from-the surface layer, it is not uncommon for an atom beneath the surface to eject from a disrupted environment and end up with a high excitation probability. This model improves upon a previous one, where the lifetime was assumed to vary with the height above the original surface.
引用
收藏
页码:8437 / 8443
页数:7
相关论文
共 26 条
[1]   ANGLE-RESOLVED VELOCITY DISTRIBUTIONS OF EXCITED RH ATOMS EJECTED FROM ION-BOMBARDED RH(100) [J].
BERNARDO, DN ;
ELMAAZAWI, M ;
MABOUDIAN, R ;
POSTAWA, Z ;
WINOGRAD, N ;
GARRISON, BJ .
JOURNAL OF CHEMICAL PHYSICS, 1992, 97 (05) :3846-3854
[2]  
BERNARDO DN, IN PRESS COMPUT PHYS
[3]  
BLANDIN A, 1976, J PHYS, V37, P396
[4]   CHARGE-EXCHANGE IN ATOM-SURFACE SCATTERING - THERMAL VERSUS QUANTUM-MECHANICAL NON-ADIABATICITY [J].
BRAKO, R ;
NEWNS, DM .
SURFACE SCIENCE, 1981, 108 (02) :253-270
[5]   EMBEDDED-ATOM METHOD - DERIVATION AND APPLICATION TO IMPURITIES, SURFACES, AND OTHER DEFECTS IN METALS [J].
DAW, MS ;
BASKES, MI .
PHYSICAL REVIEW B, 1984, 29 (12) :6443-6453
[6]   SEMIEMPIRICAL, QUANTUM-MECHANICAL CALCULATION OF HYDROGEN EMBRITTLEMENT IN METALS [J].
DAW, MS ;
BASKES, MI .
PHYSICAL REVIEW LETTERS, 1983, 50 (17) :1285-1288
[7]   INTERPRETATION OF AR+-AR COLLISIONS AT 50 KEV [J].
FANO, U ;
LICHTEN, W .
PHYSICAL REVIEW LETTERS, 1965, 14 (16) :627-&
[8]  
FOILES SM, 1986, PHYS REV B, V33, P7983, DOI 10.1103/PhysRevB.33.7983
[9]   THEORY OF AUGER EJECTION OF ELECTRONS FROM METALS BY IONS [J].
HAGSTRUM, HD .
PHYSICAL REVIEW, 1954, 96 (02) :336-365
[10]   APPLICATION OF MOLECULAR-DYNAMICS SIMULATIONS TO THE STUDY OF ION-BOMBARDED METAL-SURFACES [J].
HARRISON, DE .
CRC CRITICAL REVIEWS IN SOLID STATE AND MATERIALS SCIENCES, 1988, 14 :S1-S78