A SEDIMENT HISTORY OF SELLAFIELD DISCHARGES

被引:58
作者
KERSHAW, PJ
WOODHEAD, DS
MALCOLM, SJ
ALLINGTON, DJ
LOVETT, MB
机构
[1] Ministry of Agriculture, Fisheries and Food, Dicrectorate of Fisheries Research, Lowestoft
关键词
D O I
10.1016/0265-931X(90)90024-P
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
A suite of artificial radionuclides, discharged from the BNFL Sellafield works into the Irish Sea, has been measured in sediment cores taken from a nearby disused and undisturbed dock basin (Senhouse Dock, Maryport). This has provided a comprehensive record of Sellafield discharges from the early 1960s, including radionuclides for which discharge data are in incomplete A chronology was established by comparing a variety of radionuclide concentrations and isotope ratios in the core with the available information on decay-corrected discharges. This allowed an estimate to be made of the quantity of 238Pu discharged in the period 1959-1977 (94 ± 8 TBq) for which no discharge data exist. The transit time from discharge to incorporation in the surface sediment was in the order of 1-1·.5 y. Attempts to verify the sediment chronology with conventional 210Pbexcess dating met with difficulties because of uncertainties in the flux of 210Pb, linked to a local, anthropogenic source of 210Pb/226Ra. © 1990.
引用
收藏
页码:201 / 241
页数:41
相关论文
共 69 条
  • [1] Aston, Stanners, Observations on the deposition, mobility and chemical associations of plutonium in intertidal sediments, Techniques for Identifying Transuranics Speciation in Aquatic Environments, (1981)
  • [2] Aston, Stanners, The transport to and deposition of americium in intertidal sediments of the Ravenglass Estuary and its relationship to plutonium, Env. Poll. (Series B), 3, pp. 1-9, (1982)
  • [3] Aston, Assinder, Kelly, Plutonium in intertidal coastal and estuarine sediments in the northern Irish Sea, Est. Coast. Shelf Sci., 20, (1985)
  • [4] Berner, Sulfate reduction and the rate of deposition of marine sediments, Earth Planet. Sci. Letts., 37, (1978)
  • [5] Baker, Radiochemical techniques for determining some naturally occurring radionuclides in marine environmental materials, Nucl. Inst. Methods, 223, (1984)
  • [6] Baker, Young, The determination of thorium-234/uranium-238 disequilibrium in sediments contaminated by man-made radionuclides, Internal Rep., (1989)
  • [7] Baxter, Farmer, McKinley, Swan, Jack, Evidence of the unsuitability of gravity coring for collecting sediment in pollution and sedimentation rate studies, Environ. Sci. Technol., 15, (1981)
  • [8] BNFL, Annual report of radioactive discharges and monitoring of the environment, 1976, 1977, 1978, 1979, 1980, 1981, 1982, 1983, 1984, 1985, 1986, 1987, (1977)
  • [9] Clifton, Hamilton, The application of radioisotopes in the study of estuarine sedimentary proccesses, Est. Coastal Mar. Sci., 14, (1982)
  • [10] Comans, Middelburg, Zonderhuis, Woitticz, de Lange, Das, Van Der Wijden, Mobilization of radiocaesium in pore water of lake sediments, Nature (London), 339, (1989)