DIFFUSION OF FRACTAL AGGREGATES IN THE FREE MOLECULAR REGIME

被引:41
作者
CAI, J
SORENSEN, CM
机构
[1] Department of Physics, Kansas State University, Manhattan
来源
PHYSICAL REVIEW E | 1994年 / 50卷 / 05期
关键词
D O I
10.1103/PhysRevE.50.3397
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
We use static and dynamic light scattering to determine how the diffusion coefficient of a fractal aggregate in the free molecular regime depends on its morphological properties. Our system is a carbonaceous flame soot aerosol containing fractal aggregates with Df=1.8. We find that the Epstein equation for the diffusion coefficient holds with an effective mobility radius given by Rm=0.99aN0.43, where N is the number of monomers per aggregate and a is the monomer radius. This result is quantitatively explained as due to the projectional area of the aggregate which includes monomer-monomer screening. © 1994 The American Physical Society.
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收藏
页码:3397 / 3400
页数:4
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