MAGNETIC-PROPERTIES OF FE2NA3(PO4)3 .1. CALCULATION OF MAGNON DISPERSION-CURVES IN A COMPLEX STRUCTURE

被引:3
作者
FANJAT, N
LUCAZEAU, G
机构
[1] INST MAX VON LAUE PAUL LANGEVIN,F-38042 GRENOBLE,FRANCE
[2] ENSEEG,ION & ELECTROCHIM SOLIDE LAB,F-38402 ST MARTIN DHERES,FRANCE
关键词
MAGNONS; ANTI-FERROMAGNETISM; SUPER-SUPER-EXCHANGES; MAGNETIC FRUSTRATION;
D O I
10.1016/0022-3697(93)90307-D
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A model capable of reproducing the magnon excitations observable in the anti-ferromagnetic phase of Fe2Na3(PO4)3 is proposed. This model takes into account all the super-super-exchange interactions between the spins of the four Fe3+ of the unit cell and the neighboring spins. It is assumed that spins are collinear. The calculation method of the magnon dispersion curves is based on Saenz's formalism, and the analytical derivation of the magnon energies is performed for ideal hexagonal symmetry. Numerical calculations of magnon dispersion curves and spin deviations vs exchange interactions are reported, both in the hexagonal and triclinic symmetries. It appears that four modes can be distinguished in the triclinic symmetry. Magnetic structure stability considerations demonstrate that exchange interaction frustrations are consistent with the anti-ferromagnetic structure of the compound; it is shown that magnon dispersion curves are strongly dependent on the presence of frustrated exchange interactions.
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页码:187 / 196
页数:10
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