THE EFFECT OF 3-BODY INTERACTIONS ON THERMAL-DESORPTION SPECTRA

被引:12
作者
MYSHLYAVTSEV, AV
SALES, JL
ZGRABLICH, G
ZHDANOV, VP
机构
[1] INST CATALYSIS,NOVOSIBIRSK 630090,USSR
[2] INST INVEST TECHNOL QUIM,RA-5700 SAN LUIS,ARGENTINA
关键词
lateral interactions; Lattice-gas model; Monte Carlo simulation; transfer-matrix technique;
D O I
10.1007/BF01026561
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Thermal desorption spectra are calculated for a one-dimensional chain and for a two-dimensional square lattice using the transfer-matrix technique and Monte Carlo simulations. Lateral interactions of adsorbed particles cause a splitting of spectra. The repulsive three-body interactions are shown to lead to an inequality of the integral intensities of the thermal desorption peaks. © 1990 Plenum Publishing Corporation.
引用
收藏
页码:1029 / 1039
页数:11
相关论文
共 37 条
[1]   CONSEQUENCES OF ADSORBATE-ADSORBATE INTERACTIONS FOR THERMAL DESORPTION AND LEED MEASUREMENTS [J].
ADAMS, DL .
SURFACE SCIENCE, 1974, 42 (01) :12-36
[2]  
Baxter R. J., 2007, EXACTLY SOLVED MODEL
[3]   INFLUENCE OF ADSORBATE INTERACTIONS ON HETEROGENEOUS REACTION-KINETICS - FORMIC-ACID DECOMPOSITION ON NICKEL [J].
BENZIGER, JB ;
SCHOOFS, GR .
JOURNAL OF PHYSICAL CHEMISTRY, 1984, 88 (19) :4439-4444
[4]  
BINDER K, 1981, SURF SCI, V108, P2503
[5]   ASSOCIATIVE DESORPTION FROM ADLAYERS OF INTERACTING PARTICLES - NITRIC-OXIDE ON PT, NI AND RU [J].
BRIDGE, ME ;
LAMBERT, RM .
PROCEEDINGS OF THE ROYAL SOCIETY OF LONDON SERIES A-MATHEMATICAL AND PHYSICAL SCIENCES, 1980, 370 (1743) :545-560
[6]   ADSORPTION AND REACTIVITY OF NITRIC-OXIDE ON CO(0001) [J].
BRIDGE, ME ;
LAMBERT, RM .
SURFACE SCIENCE, 1980, 94 (2-3) :469-482
[7]   DESORPTION FROM NON-EQUILIBRIUM ISLAND-FORMING ADLAYERS [J].
EVANS, JW ;
PAK, H .
SURFACE SCIENCE, 1988, 199 (1-2) :28-42
[8]   DESORPTION FROM AN IMMOBILE ADLAYER - EXACT ONE-DIMENSIONAL KINETICS [J].
EVANS, JW ;
HOFFMAN, DK ;
PAK, H .
SURFACE SCIENCE, 1987, 192 (2-3) :475-490
[9]   MONTE-CARLO SIMULATION OF TEMPERATURE-PROGRAMMED DESORPTION OF MOLECULES FROM SOLID-SURFACES [J].
GUPTA, D ;
HIRTZEL, CS .
CHEMICAL PHYSICS LETTERS, 1988, 149 (5-6) :527-533
[10]   THERMAL-DESORPTION OF INTERACTING MOLECULES FROM MIXED ADLAYERS [J].
GUPTA, D ;
HIRTZEL, CS .
SURFACE SCIENCE, 1989, 210 (03) :322-338