METASTABLE IMPURITY-HELIUM SOLID-PHASE - EXPERIMENTAL AND THEORETICAL EVIDENCE

被引:54
作者
GORDON, EB [1 ]
KHMELENKO, VV [1 ]
PELMENEV, AA [1 ]
POPOV, EA [1 ]
PUGACHEV, OF [1 ]
SHESTAKOV, AF [1 ]
机构
[1] RUSSIAN ACAD SCI,INST CHEM PHYS,CHERNOGOLOVKA 142432,RUSSIA
关键词
D O I
10.1016/0301-0104(93)85122-O
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A novel solid metastable phase of ''sticking-together'' helium van der Waals coats surrounding polarizable heavy impurities - Ne, Ar, Kr, Xe, N and N2 - has been obtained and investigated using the experimental technique based on ps beam injection into superfluid helium. The element composition for this phase was measured and for all inert gases the solid samples were found to consist of more than 90% helium atoms and to keep stability up to T almost-equal-to 8 K. The cluster approach to the theoretical analysis of the model NeHe12 Structures developed makes it possible to suggest the main physical reason for its formation to be the breakdown of quantum-mechanical helium atoms behavior, namely, strong suppression of amplitudes of radial zeroth vibrations for helium atoms belonging to the van der Waals shell in the field of dispersion forces of the central impurity particle. The phase diagram for the impurity-helium substance has been simulated and the directions of future investigations have also been outlined.
引用
收藏
页码:411 / 426
页数:16
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