ACIDITY AND STABILITY OF MCM-41 CRYSTALLINE ALUMINOSILICATES

被引:639
作者
CORMA, A
FORNES, V
NAVARRO, MT
PEREZPARIENTE, J
机构
[1] Institute de Tecnología Química, U.P.V.-C.S-I.C., Universidad Politécnica, 46071 Valencia, Cno. de Vera. S/n
关键词
D O I
10.1006/jcat.1994.1243
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
MCM-41 samples with different Si/Al ratios have been synthesized, and their stability and acidity characteristics have been studied. It has been shown that MCM-41 is readily dealuminated upon thermal treatment both in air and in N2 atmosphere. After calcination the sample shows an acidity of medium strength as compared with a USY zeolite. Calcination in N2 atmosphere leads to samples with better textural and acid characteristics. (C) 1994 Academic Press, Inc.
引用
收藏
页码:569 / 574
页数:6
相关论文
共 14 条
[1]   A NEW FAMILY OF MESOPOROUS MOLECULAR-SIEVES PREPARED WITH LIQUID-CRYSTAL TEMPLATES [J].
BECK, JS ;
VARTULI, JC ;
ROTH, WJ ;
LEONOWICZ, ME ;
KRESGE, CT ;
SCHMITT, KD ;
CHU, CTW ;
OLSON, DH ;
SHEPPARD, EW ;
MCCULLEN, SB ;
HIGGINS, JB ;
SCHLENKER, JL .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1992, 114 (27) :10834-10843
[2]   STUDIES ON MESOPOROUS MATERIALS .1. SYNTHESIS AND CHARACTERIZATION OF MCM-41 [J].
CHEN, CY ;
LI, HX ;
DAVIS, ME .
MICROPOROUS MATERIALS, 1993, 2 (01) :17-26
[3]  
CORMA A, 1990, APPL CATAL, V59, P261
[4]  
CORMA A, 1991, ACS SYM SER, V452, P79
[5]   A MOLECULAR-SIEVE WITH 18-MEMBERED RINGS [J].
DAVIS, ME ;
SALDARRIAGA, C ;
MONTES, C ;
GARCES, J ;
CROWDER, C .
NATURE, 1988, 331 (6158) :698-699
[6]   A SYNTHETIC GALLOPHOSPHATE MOLECULAR-SIEVE WITH A 20-TETRAHEDRAL-ATOM PORE OPENING [J].
ESTERMANN, M ;
MCCUSKER, LB ;
BAERLOCHER, C ;
MERROUCHE, A ;
KESSLER, H .
NATURE, 1991, 352 (6333) :320-323
[7]   PILLARED CLAYS AS CATALYSTS [J].
FIGUERAS, F .
CATALYSIS REVIEWS-SCIENCE AND ENGINEERING, 1988, 30 (03) :457-499
[8]   METHOD FOR THE CALCULATION OF EFFECTIVE PORE-SIZE DISTRIBUTION IN MOLECULAR-SIEVE CARBON [J].
HORVATH, G ;
KAWAZOE, K .
JOURNAL OF CHEMICAL ENGINEERING OF JAPAN, 1983, 16 (06) :470-475
[9]   A STUDY OF SURFACE STRUCTURE OF DECATIONIZED Y ZEOLITE BY QUANTITATIVE INFRARED SPECTROSCOPY [J].
HUGHES, TR ;
WHITE, HM .
JOURNAL OF PHYSICAL CHEMISTRY, 1967, 71 (07) :2192-&
[10]  
JACOBS PA, 1984, J CATAL, V22, P193