SOL-GEL PROCESSING AND MICROWAVE CHARACTERISTICS OF BA(MG1/3TA2/3)O3 DIELECTRICS

被引:74
作者
RENOULT, O [1 ]
BOILOT, JP [1 ]
CHAPUT, F [1 ]
PAPIERNIK, R [1 ]
HUBERTPFLALZGRAF, LG [1 ]
LEJEUNE, M [1 ]
机构
[1] UNIV NICE,CHIM MOLEC LAB,F-06034 NICE,FRANCE
关键词
D O I
10.1111/j.1151-2916.1992.tb04430.x
中图分类号
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
The sol-gel method has been developed for the preparation of pure Ba(Mg1/3Ta2/3)O3 ceramics. This involves the reaction of the heterometallic alkoxide Ta2Mg(OEt)12 with hydrated barium hydroxide Ba(OH)2-8H2O. Complete crystallization of the sol-gel-derived powder is achieved at 600-degrees-C, leading to a cubic perovskite type phase. After sintering at 1400-degrees-C (2-5 h), a trigonal cell arises from Mg-Ta ordering (the degree of order is greater than 0.9), and about 98.5% of the theoretical density is obtained. Preliminary microwave dielectric measurements show that the dielectric constant and the unloaded Q(u) of the ceramics are 24.2 and 6750, respectively, at 7.7 GHz.
引用
收藏
页码:3337 / 3340
页数:4
相关论文
共 17 条
[1]   DIELECTRIC-PROPERTIES OF SR(NI1/3NB2/3)O3-BA(NI1/3NB2/3)O3 CERAMICS AT MICROWAVE-FREQUENCIES [J].
BANNO, H ;
MIZUNO, F ;
TAKEUCHI, T ;
TSUNOOKA, T ;
OHYA, K .
JAPANESE JOURNAL OF APPLIED PHYSICS PART 1-REGULAR PAPERS SHORT NOTES & REVIEW PAPERS, 1985, 24 :87-89
[2]   STRUCTURAL CHEMISTRY OF THE ALKOXIDES .8. ISOMERIC BUTOXIDES AND PENTYLOXIDES OF NIOBIUM [J].
BRADLEY, DC ;
CHAKRAVARTI, BN ;
WARDLAW, W .
JOURNAL OF THE CHEMICAL SOCIETY, 1956, (NOV) :4439-4442
[3]   ALKOXIDE HYDROXIDE ROUTE TO SYNTHESIZE BATIO3-BASED POWDERS [J].
CHAPUT, F ;
BOILOT, JP ;
BEAUGER, A .
JOURNAL OF THE AMERICAN CERAMIC SOCIETY, 1990, 73 (04) :942-948
[4]   LOW-TEMPERATURE ROUTE TO LEAD MAGNESIUM NIOBATE [J].
CHAPUT, F ;
BOILOT, JP ;
LEJEUNE, M ;
PAPIERNIK, R ;
HUBERTPFALZGRAF, LG .
JOURNAL OF THE AMERICAN CERAMIC SOCIETY, 1989, 72 (08) :1355-1357
[5]   MICROWAVE LOSS QUALITY OF BAZN1/3TA2/3O3 CERAMICS [J].
DESU, SB ;
OBRYAN, HM .
JOURNAL OF THE AMERICAN CERAMIC SOCIETY, 1985, 68 (10) :546-551
[6]   ORDERING IN COMPOUNDS OF A(B'0.33TA0.67)O3TYPE [J].
GALASSO, F ;
PYLE, J .
INORGANIC CHEMISTRY, 1963, 2 (03) :482-&
[7]  
Hakki BW, 1960, IRE T MICROWAVE THEO, V8, P402, DOI DOI 10.1109/TMTT.1960.1124749
[8]  
HENNINGS D, 1983, PHILIPS J RES, V38, P295
[9]   BA(ZN1/3TA2/3)O-3 CERAMICS WITH LOW DIELECTRIC LOSS AT MICROWAVE-FREQUENCIES [J].
KAWASHIMA, S ;
NISHIDA, M ;
UEDA, I ;
OUCHI, H .
JOURNAL OF THE AMERICAN CERAMIC SOCIETY, 1983, 66 (06) :421-423
[10]  
MATSUMOTO K, 1986, 6TH P IEEE INT S APP, P118