RELAXATION PHENOMENA IN SELF-ASSEMBLED SYSTEMS

被引:8
作者
LEVIN, Y
MUNDY, CJ
DAWSON, KA
机构
[1] UNIV CALIF BERKELEY,DEPT CHEM,BERKELEY,CA 94720
[2] NATL UNIV IRELAND UNIV COLL DUBLIN,DEPT CHEM,DUBLIN 4,IRELAND
来源
PHYSICA A | 1993年 / 196卷 / 02期
关键词
D O I
10.1016/0378-4371(93)90599-Y
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
A dynamical model is proposed to study the evolution of the structure factor in the isotropic phase of a frustrated spin model. The study has application to the development of structure in bicontinuous microemulsions. We consider both non-conserved order parameters (NCOP) and the conserved order parameters (COP). In the former case (NCOP), within a self-consistent meanfield theory, we find that in the asymptotic limit (t --> infinity) all modes of the structure factor decay with the same characteristic time. This characteristic time scales with the two fundamental lengths d and xi is present in self-assembled systems such as frustrated magnetic systems and binary alloys. In the latter case (COP), we find that no characteristic time is present within self-consistent mean-field theory and all modes decay algebraically. This is reminiscent of the long time tails in the velocity-velocity autocorrelation function observed for simple fluids.
引用
收藏
页码:173 / 187
页数:15
相关论文
共 38 条
[1]   VELOCITY AUTOCORRELATIONS FOR HARD SPHERES [J].
ALDER, BJ ;
WAINWRIGHT, TE .
PHYSICAL REVIEW LETTERS, 1967, 18 (23) :988-+
[2]  
BARBOSA MC, PREPRINT
[3]   LOW-TEMPERATURE EXPANSION OF A SPATIALLY FRUSTRATED ISOTROPIC LATTICE MODEL [J].
BERERA, A ;
DAWSON, KA .
PHYSICAL REVIEW A, 1990, 41 (02) :626-643
[4]  
BRAZOVSKII SA, 1978, SOLID STATE PHYS, V41, P85
[5]  
BRENIG W, 1989, STATISTICAL THEORY H
[6]   MICROEMULSIONS IN OIL-WATER-SURFACTANT MIXTURES - SYSTEMATICS OF A LATTICE-GAS MODEL [J].
CHEN, K ;
EBNER, C ;
JAYAPRAKASH, C ;
PANDIT, R .
PHYSICAL REVIEW A, 1988, 38 (12) :6240-6254
[7]  
CHEN K, 1987, J PHYS C SOLID STATE, V20, P1361
[8]   MICROSCOPIC MODEL FOR MICROEMULSIONS .2. BEHAVIOR AT LOW-TEMPERATURES AND CRITICAL-POINT [J].
CIACH, A ;
HOYE, JS .
JOURNAL OF CHEMICAL PHYSICS, 1989, 90 (02) :1222-1228
[9]   MICROSCOPIC MODEL FOR MICROEMULSIONS .1. GROUND-STATE PROPERTIES [J].
CIACH, A ;
HOYE, JS ;
STELL, G .
JOURNAL OF CHEMICAL PHYSICS, 1989, 90 (02) :1214-1221
[10]  
CIACH A, 1989, J PHYS A, V21, P777