PHASE-CONTROL IN THE 2-COLOR PHOTODISSOCIATION OF HD+

被引：247

作者：

SHEEHY, B

WALKER, B

DIMAURO, LF

机构：

[1] Chemistry Department, Brookhaven National Laboratory, Upton

来源：

PHYSICAL REVIEW LETTERS | 1995年 / 74卷 / 24期

关键词：

D O I：

10.1103/PhysRevLett.74.4799

中图分类号：

O4 [物理学];

学科分类号：

0702 ;

摘要：

We report on the use of the relative phase between a two-color optical field (1053 and 527 nm) to coherently control the photodissociation of the HD+ molecule. The field-induced spatial asymmetry in the fragment spectrum shows a strong phase dependence, while no selectivity is produced in nearly isoenergetic channels. The positively charged fragments are observed to preferentially dissociate in a direction counterintuitive to classical expectations. © 1995 The American Physical Society.

引用

页码：4799 / 4802

页数：4

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