HIGH-PRESSURE LOW-TEMPERATURE OPTICAL DEPHASING OF RHODAMINE-101 IN PMMA

被引:18
作者
BAER, BJ [1 ]
CROWELL, RA [1 ]
CHRONISTER, EL [1 ]
机构
[1] UNIV CALIF RIVERSIDE,DEPT CHEM,RIVERSIDE,CA 92521
基金
美国国家科学基金会;
关键词
D O I
10.1016/0009-2614(95)00312-R
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
High pressure (0-30 kbar) is used to investigate the effect of increased density on the temperature-dependent optical dephasing of rhodamine 101 (Rh101) in polymethyl methacrylate (PMMA). Photon echo measurements have been performed on Rh101-doped PMMA at temperatures between 1.2 and 2.1 K at pressures up to 30 kbar. The 20% volume compression at 30 kbar resulted in little change in either the magnitude or the temperature dependence of the optical dephasing rate. The pressure insensitive homogeneous linewidth Gamma = 110 T-1.35 MHz is discussed in terms of the two level system model often used to characterize the optical dynamics of glasses.
引用
收藏
页码:380 / 386
页数:7
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