2-COLOR COHERENT CONTROL WITH SEP PREPARATION - ELECTRONIC BRANCHING IN NA-2 PHOTODISSOCIATION

被引：4

作者：

DODS, J

BRUMER, P

SHAPIRO, M

机构：

[1] UNIV TORONTO,DEPT CHEM,CHEM PHYS THEORY GRP,TORONTO M5S 1A1,ON,CANADA

[2] WEIZMANN INST SCI,DEPT CHEM PHYS,IL-76100 REHOVOT,ISRAEL

来源：

CANADIAN JOURNAL OF CHEMISTRY-REVUE CANADIENNE DE CHIMIE | 1994年 / 72卷 / 03期

关键词：

D O I：

10.1139/v94-124

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Extensive control over relative product yields is shown to result from weak laser photodissociation in a two-color coherent control scenario. Photodissociation takes place from a superposition state prepared by stimulated emission pumping. The method allows for control in the presence of laser phase jumps by using four-wave mixing to prepare the required laser frequencies. The near W photodissociation of Na-2, resulting in the Na(3s) + Na(4s) and the Na(Ss) + Na(3d) products, is used to illustrate the method.

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页码：958 / 965

页数：8

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