A MICRO-PHYSICAL BOX MODEL FOR EASOE - PRELIMINARY-RESULTS FOR THE JANUARY FEBRUARY 1990 PSC EVENT OVER KIRUNA

被引:9
作者
PETER, T
MULLER, R
DRDLA, K
PETZOLDT, K
REIMER, E
机构
[1] UNIV CALIF LOS ANGELES, DEPT ATMOSPHER SCI, LOS ANGELES, CA 90024 USA
[2] FREE UNIV BERLIN, INST METEOROL, W-1000 BERLIN 41, GERMANY
来源
BERICHTE DER BUNSEN-GESELLSCHAFT-PHYSICAL CHEMISTRY CHEMICAL PHYSICS | 1992年 / 96卷 / 03期
关键词
ATMOSPHERIC AEROSOLS; CRYSTAL GROWTH; NUCLEATION;
D O I
10.1002/bbpc.19920960324
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
First results of a trajectory box model designed for the European Arctic Stratospheric Ozone Experiment (EASOE) are presented. The model contains a comprehensive description of both types of polar stratospheric particles, NAT on aerosol (Type-I) and ice on NAT (Type-II), including nucleation, growth/evaporation, and sedimentation of particles. The performance of the model is tested for the case of the polar stratospheric cloud (PSC) event January 31-February 1, 1990 over Kiruna (north Sweden). Comparison of the model results with measurements from two stratospheric balloon flights shows that the theory can reproduce the data provided the following two conditions are satisfied: (a) a strong lee wave activity was present at the time of the balloon flights; (b) the nucleation of NAT on H2SO4 is either governed by a high barrier energy or delayed due to insufficient freezing of the background aerosol. These results indicate an urgent need for both, the implementation of lee wave effects into the existing trajectory models and a better understanding of the NAT nucleation on the background aerosol.
引用
收藏
页码:362 / 367
页数:6
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