SURFACE-DIFFUSION ON HETEROGENEOUS CORRELATED SUBSTRATES

被引:8
作者
BULNES, F [1 ]
RICCARDO, JL [1 ]
ZGRABLICH, G [1 ]
PEREYRA, V [1 ]
机构
[1] UNIV NACL SAN LUIS,CONSEJO NACL INVEST CIENT & TECN,INST INVEST TECNOL QUIM,CASILLA CORREO 290,RA-5700 SAN LUIS,ARGENTINA
关键词
D O I
10.1016/0039-6028(92)90045-8
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The behaviour of the surface diffusion coefficient on an heterogeneous correlated surface is studied in the framework of the lattice-gas model. Using the multivariate adsorptive energy distribution function the statistical properties of the heterogeneous correlated surface can be appropriately described and the effect of the heterogeneity on the collective diffusion coefficient at finite coverage can be analized through a correlation length. Monte Carlo simulation is also performed to test the analytical results.
引用
收藏
页码:304 / 310
页数:7
相关论文
共 21 条
[1]  
[Anonymous], 1974, INTERACTION GASES SO
[2]  
HAUS JW, 1987, PHYS REP, V150, P264
[3]  
HAUS JW, 1982, PHYS REV B, V25, P290
[4]   MONTE-CARLO SIMULATIONS OF INTERSTITIAL DIFFUSION AND TRAPPING .2. AMORPHOUS METALS [J].
KIRCHHEIM, R ;
STOLZ, U .
ACTA METALLURGICA, 1987, 35 (02) :281-291
[5]   MONTE-CARLO STUDIES OF DIFFUSION ON INHOMOGENEOUS SURFACES [J].
MAK, CH ;
ANDERSEN, HC ;
GEORGE, SM .
JOURNAL OF CHEMICAL PHYSICS, 1988, 88 (06) :4052-4061
[6]   DUAL SITE-BOND DESCRIPTION OF HETEROGENEOUS SURFACES [J].
MAYAGOITIA, V ;
ROJAS, F ;
RICCARDO, JL ;
PEREYRA, VD ;
ZGRABLICH, G .
PHYSICAL REVIEW B, 1990, 41 (10) :7150-7155
[7]   MECHANISTIC STUDY OF SURFACE PROCESSES ON ADSORBENTS .1. STATISTICAL DESCRIPTION OF ADSORPTIVE SURFACES [J].
MAYAGOITIA, V ;
ROJAS, F ;
PEREYRA, VD ;
ZGRABLICH, G .
SURFACE SCIENCE, 1989, 221 (1-2) :394-408
[8]   SURFACE-DIFFUSION OF ADSORBED GASES AS A PERCOLATION PROCESS [J].
PEREYRA, V ;
ZGRABLICH, G .
SURFACE SCIENCE, 1989, 209 (03) :512-522
[9]   A BASIC APPROACH TO SURFACE-DIFFUSION ON HETEROGENEOUS SUBSTRATES [J].
PEREYRA, V ;
ZGRABLICH, G .
LANGMUIR, 1990, 6 (01) :118-121
[10]   GENERAL EQUATIONS FOR DESCRIBING DIFFUSION ON THE HETEROGENEOUS SURFACE AT FINITE COVERAGES [J].
PEREYRA, V ;
ZGRABLICH, G ;
ZHDANOV, VP .
LANGMUIR, 1990, 6 (03) :691-694