A NEUTRON-DIFFRACTION STUDY OF ACID SITES IN H-SAPO-37

被引:15
作者
BULL, LM
CHEETHAM, AK
HOPKINS, PD
POWELL, BM
机构
[1] AMOCO OIL CO,AMOCO RES CTR,NAPERVILLE,IL 60566
[2] AECL RES,CHALK RIVER LAB,CHALK RIVER,ON,CANADA
关键词
D O I
10.1039/c39930001196
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A powder neutron diffraction study of H-SAPO-37 (Fd3; a = 24.804(2) angstrom; R(p) = 2.98%, R(wp) = 3.73%, chi2 = 1.966) reveals Al/P alternation in the framework, with Si substituting for P; protonation, in order of decreasing occupancy, is observed at O(1), O(2) and O(3).
引用
收藏
页码:1196 / 1198
页数:3
相关论文
共 16 条
[1]  
BENNETT JM, 1983, ACS SYM SER, V218, P109
[2]  
BLASCO T, 1993, 9TH P INT ZEOL C MON
[3]   THERMAL AND HYDROTHERMAL STABILITY OF SAPO-5 AND SAPO-37 MOLECULAR-SIEVES [J].
BRIEND, M ;
SHIKHOLESLAMI, A ;
PELTRE, MJ ;
DELAFOSSE, D ;
BARTHOMEUF, D .
JOURNAL OF THE CHEMICAL SOCIETY-DALTON TRANSACTIONS, 1989, (07) :1361-1362
[4]   THE DIRECT OBSERVATION OF CATION HYDROLYSIS IN LANTHANUM ZEOLITE-Y BY NEUTRON-DIFFRACTION [J].
CHEETHAM, AK ;
EDDY, MM ;
THOMAS, JM .
JOURNAL OF THE CHEMICAL SOCIETY-CHEMICAL COMMUNICATIONS, 1984, (20) :1337-1338
[5]   DIRECT DETERMINATION OF PROTON POSITIONS IN D-Y AND H-Y ZEOLITE SAMPLES BY NEUTRON POWDER DIFFRACTION [J].
CZJZEK, M ;
JOBIC, H ;
FITCH, AN ;
VOGT, T .
JOURNAL OF PHYSICAL CHEMISTRY, 1992, 96 (04) :1535-1540
[6]   THE ACIDIC PROPERTIES OF SAPO-37 COMPARED TO FAUJASITES AND SAPO-5 [J].
DZWIGAJ, S ;
BRIEND, M ;
SHIKHOLESLAMI, A ;
PELTRE, MJ ;
BARTHOMEUF, D .
ZEOLITES, 1990, 10 (03) :157-162
[7]   ALUMINOPHOSPHATE MOLECULAR-SIEVES AND THE PERIODIC-TABLE [J].
FLANIGEN, EM ;
LOK, BM ;
PATTON, RL ;
WILSON, ST .
PURE AND APPLIED CHEMISTRY, 1986, 58 (10) :1351-1358
[8]  
Gibbs G. V., 1977, ACS SYM SER, V40, P19
[9]  
Habib T.E., 1979, FLUID CATALYTIC CRAC
[10]   ASSIGNMENT OF HYDROXYL BANDS IN INFRARED-SPECTRA OF ZEOLITES X AND Y .1. NA - H ZEOLITES [J].
JACOBS, PA ;
UYTTERHOEVEN, JB .
JOURNAL OF THE CHEMICAL SOCIETY-FARADAY TRANSACTIONS I, 1973, 69 (02) :359-372