LASER-NOISE-INDUCED POLARIZATION FLUCTUATIONS AS A SPECTROSCOPIC TOOL

We have investigated theoretically the possibility of employing noisy laser fields for spectroscopic purposes. The basis for this spectroscopy is a modification of the statistic of the fluctuations caused by the nonlinear interaction. All atomic resonances within the range of several bandwidths can be observed in the power spectrum, even in case of large inhomogeneous broadening. We have derived analytical, nonperturbative results for a real Gaussian, a complex Gaussian, and a phase-diffusing field. The mean transmitted intensity and its variance as well as the power spectrum have been evaluated in the limit of weak absorption for two-level systems. Without modification, we can apply our results also to other transition schemes. As an example, the power spectrum of the D2 transition of Cs-133 driven by a phase-diffusing field is calculated. For this four-level system we find qualitative agreement with experimental results by Yabuzaki et al. [Phys. Rev. Lett. 67, 2453 (1991)].