LASER SPECTROSCOPY OF ALKALI-DOPED HELIUM CLUSTERS

被引：155

作者：

STIENKEMEIER, F

HIGGINS, J

ERNST, WE

SCOLES, G

机构：

[1] PENN STATE UNIV, DEPT PHYS, UNIVERSITY PK, PA 16802 USA

[2] PRINCETON UNIV, DEPT CHEM, PRINCETON, NJ 08544 USA

来源：

PHYSICAL REVIEW LETTERS | 1995年 / 74卷 / 18期

关键词：

D O I：

10.1103/PhysRevLett.74.3592

中图分类号：

O4 [物理学];

学科分类号：

0702 ;

摘要：

A beam of HeN clusters (103N104) is seeded with one or more chromophores by sticky collisions with a low pressure gas and is probed, thereafter, by laser-induced fluorescence spectroscopy. Using sodium, we observe the spectra of atoms, dimers, and trimers and find that they are almost unshifted from their gas phase counterparts, but show cluster-induced broadenings in the range of tens of cm-1. Upon formation on the cluster surface, a fraction of the dimers desorbs slowly and becomes part of the beam, allowing narrow, rotationally resolved, spectra to be obtained. © 1995 The American Physical Society.

引用

页码：3592 / 3595

页数：4

共 34 条

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