THE TEMPORAL AND SPATIAL VARIABILITY OF SCAVENGING RATIOS FOR NSS SULFATE, NITRATE, METHANESULFONATE AND SODIUM IN THE ATMOSPHERE OVER THE NORTH-ATLANTIC OCEAN

被引：107

作者：

GALLOWAY, JN ^{[1
]}

SAVOIE, DL ^{[1
]}

KEENE, WC ^{[1
]}

PROSPERO, JM ^{[1
]}

机构：

[1] UNIV MIAMI,DIV MARINE & ATMOSPHER CHEM,MIAMI,FL 33149

来源：

ATMOSPHERIC ENVIRONMENT PART A-GENERAL TOPICS | 1993年 / 27卷 / 02期

关键词：

AEROSOL; PRECIPITATION; MARINE ATMOSPHERE; SCAVENGING RATIO; WASHOUT RATIO; WET DEPOSITION; ATMOSPHERIC CHEMISTRY; SULFATE; NITRATE; SODIUM; METHANESULFONATE;

D O I：

10.1016/0960-1686(93)90354-2

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

In this paper we study the temporal and spatial variability of scavenging ratios (SRs) based upon 2 years of continuous aerosol and precipitation data collected at three sites of the Atmosphere-Ocean Chemistry Experiment (AEROCE): Barbados, Bermuda and Ireland. At Barbados and Bermuda, the SRs for nss SO42-, NO3- and CH3SO3- fell within a relatively narrow range: 210-374; for the individual species, the absolute differences between the two site means were quite small, ranging from 9% for NO3-, to 36% for CH3SO3-. SRs at Ireland were very different but the situation is complicated due to the sectoring of aerosol but not of precipitation. On shorter time scales (days to months), SRs are highly variable and can range over orders of magnitude. Consequently, SRs based on short-term measurements at one place and time should be used with caution at other places and times. Nonetheless. the similarity in our 2-year mean SRs at Barbados and Bermuda suggests that SRs might be relatively constant over longer time periods.

引用

页码：235 / 250

页数：16

共 39 条

[1] ATMOSPHERIC TRACE-ELEMENTS AT ENEWETAK ATOLL .2. TRANSPORT TO THE OCEAN BY WET AND DRY DEPOSITION [J].

ARIMOTO, R ;

DUCE, RA ;

RAY, BJ ;

UNNI, CK .

JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1985, 90 (ND1) :2391-2408

[2] A TECHNIQUE USING HIGH- FLOW, DICHOTOblOUS FILTER PACKS FOR MEASURING MAJOR ATMOSPHERIC CHEMICAL CONSTITUENTS [J].

Bardwell, C. ;

Maben, J. ;

Hurt, J. ;

Keene, W. ;

Galloway, J. ;

Boatman, I. ;

Wellman, D. .

GLOBAL BIOGEOCHEMICAL CYCLES, 1990, 4 (02) :151-163

[3] SCAVENGING RATIOS, WET DEPOSITION, AND IN-CLOUD OXIDATION - AN APPLICATION TO THE OXIDES OF SULFUR AND NITROGEN [J].

BARRIE, LA .

JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1985, 90 (ND3) :5789-5799

[4]

BARRIE LA, 1991, 5TH P INT C PREC SCV

[5] PRECIPITATION SCAVENGING OF AEROSOL-PARTICLES OVER REMOTE MARINE REGIONS [J].

BUATMENARD, P ;

DUCE, RA .

NATURE, 1986, 321 (6069) :508-510

[6] ATMOSPHERIC AND PRECIPITATION CHEMISTRY OVER THE NORTH-ATLANTIC OCEAN - SHIPBOARD RESULTS, APRIL-MAY 1984 [J].

CHURCH, TM ;

TRAMONTANO, JM ;

WHELPDALE, DM ;

ANDREAE, MO ;

GALLOWAY, JN ;

KEENE, WC ;

KNAP, AH ;

TOKOS, J .

JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1991, 96 (D10) :18705-18725

[7] THE ATMOSPHERIC INPUT OF TRACE SPECIES TO THE WORLD OCEAN [J].

Duce, R. ;

Liss, P. ;

Merrill, J. ;

Atlas, E. ;

Buat-Menard, P. ;

Hicks, B. ;

Miller, J. ;

Prospero, J. ;

Arimoto, R. ;

Church, T. ;

Ellis, W. ;

Galloway, J. ;

Hansen, L. ;

Jickells, T. ;

Knap, A. ;

Reinhardt, K. ;

Schneider, B. ;

Soudine, A. ;

Tokos, J. ;

Tsunogai, S. ;

Wollast, R. ;

Zhou, M. .

GLOBAL BIOGEOCHEMICAL CYCLES, 1991, 5 (03) :193-259

[8] ON THE USE OF SCAVENGING RATIOS FOR THE INFERENCE OF SURFACE-LEVEL CONCENTRATIONS AND SUBSEQUENT DRY DEPOSITION OF CA2+, MG2+, NA+ AND K+ [J].

EDER, BK ;

DENNIS, RL .

WATER AIR AND SOIL POLLUTION, 1990, 52 (3-4) :197-216

[9]

ENGELMANN RJ, 1971, J APPL METEOROL, V10, P493

[10]

GATZ DF, 1974, OCT P PREC SCAV S CH

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