ONE AND 2 PHOTON SPECTRA OF SF6, MOLECULAR-BEAM MEASUREMENTS

被引:23
作者
LINSKENS, A
HEKKERT, STL
REUSS, J
机构
[1] Fysisch Laboratorium, Katholieke Universiteit Nijmegen, 6525 ED Nijmegen, Toernooiveld
来源
INFRARED PHYSICS | 1991年 / 32卷
关键词
D O I
10.1016/0020-0891(91)90116-W
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Experiments on the saturation behaviour of one and two photon transitions have been performed on a molecular beam of SF6-molecules, using single mode cw CO2-lasers. Application of an Acousto Optic Modulator allowed a total tuning range of 0.6 GHz around each CO2 laser line. Numerous, partially new absorptions have been observed and are catalogued. From the assigned transitions on the 10P16 laser line a rotational Boltzmann plot was derived showing strong deviation from a thermal distribution. Transitions from the RAP regime, with inversion, to the Rabi regime, with power broadening, have been observed, utilizing opto-thermal detection. A clear two photon Rabi oscillation has been observed.
引用
收藏
页码:259 / 282
页数:24
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