STRUCTURE INVESTIGATIONS OF XE-ADSORBATE LAYERS BY SPIN-POLARIZED LOW-ENERGY-ELECTRON DIFFRACTION .2. (ROOT-3X-ROOT-3)R30-DEGREES-XE PD(111) AND THE DILUTE PHASE OF XE PD(111)

被引:26
作者
HILGERS, G [1 ]
POTTHOFF, M [1 ]
MULLER, N [1 ]
HEINZMANN, U [1 ]
机构
[1] UNIV BIELEFELD,FAK PHYS,D-33501 BIELEFELD,GERMANY
关键词
ADATOMS; ELECTRON-SOLID INTERACTIONS; SCATTERING; DIFFRACTION; LOW ENERGY ELECTRON DIFFRACTION (LEED); LOW INDEX SINGLE CRYSTAL SURFACES; METALLIC SURFACES; PALLADIUM; SURFACE STRUCTURE; MORPHOLOGY; ROUGHNESS; AND TOPOGRAPHY;
D O I
10.1016/0039-6028(95)90031-4
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The adsorbate systems (root 3 x root 3)R30 degrees-Xe/Pd(111) and the 'dilute' phase of Xe/Pd(111) were investigated with spin-polarized low-energy electron diffraction (SPLEED). Spin-polarized electrons from a GaAs source were scattered and the spin-dependent intensities were measured. Comparative calculations were carried out by means of a relativistic LEED program. The structure determination of (root 3 x root 3)R30 degrees-Xe/Pd(111) yields a layer distance of 3.5+/-0.1 Angstrom, the Xe atoms being adsorbed in hollow sites. In the 'dilute' phase of Xe/Pd(111) the adsorbed Xe atoms occupy on-top sites with a Xe-Pd distance of 4.0+/-0.1 Angstrom without two-dimensional periodicity.
引用
收藏
页码:207 / 220
页数:14
相关论文
共 24 条
[1]   ANGLE-RESOLVED PHOTOEMISSION OF XENON ADSORBED ON PT(111) - COMMENSURATE AND INCOMMENSURATE MONOLAYERS [J].
CASSUTO, A ;
EHRHARDT, JJ .
JOURNAL DE PHYSIQUE, 1988, 49 (10) :1753-1759
[2]   DYNAMICAL THEORY OF LOW-ENERGY-ELECTRON DIFFRACTION FROM DISORDERED OVERLAYERS .2. APPLICATION TO ONE-DIMENSIONAL ADSORBATES [J].
DUKE, CB ;
LIEBSCH, A .
PHYSICAL REVIEW B, 1974, 9 (04) :1150-1159
[3]   SPIN POLARIZATION IN LOW-ENERGY ELECTRON-DIFFRACTION - SURFACE-ANALYSIS OF PT(111) [J].
FEDER, R ;
PLEYER, H ;
BAUER, P ;
MULLER, N .
SURFACE SCIENCE, 1981, 109 (02) :419-434
[4]   SPIN-POLARIZED LOW-ENERGY ELECTRON-DIFFRACTION - THEORY, EXPERIMENT AND ANALYSIS OF RESULTS FROM W(001)(1X1) [J].
FEDER, R ;
KIRSCHNER, J .
SURFACE SCIENCE, 1981, 103 (01) :75-102
[5]   STRUCTURAL INVESTIGATIONS ON XE/PD(111) WITH SPIN-POLARIZED LEED [J].
HILGERS, G ;
POTTHOFF, M ;
MULLER, N ;
HEINZMANN, U .
SURFACE SCIENCE, 1993, 287 (pt A) :414-417
[6]  
HILGERS G, 1992, THESIS U BIELEFELD
[7]   DIFFUSE LEED INTENSITIES OF DISORDERED CRYSTAL-SURFACES .1. CORRELATIONS BETWEEN STATISTICS AND MULTIPLE DIFFRACTION [J].
JAGODZINSKI, H ;
MORITZ, W ;
WOLF, D .
SURFACE SCIENCE, 1978, 77 (02) :233-248
[8]   AN EFFICIENT METHOD FOR LEED CRYSTALLOGRAPHY [J].
KLEINLE, G ;
MORITZ, W ;
ERTL, G .
SURFACE SCIENCE, 1990, 238 (1-3) :119-131
[9]   THE ADSORPTION OF SULFUR ON PD(111) .1. A LEED ANALYSIS OF THE (SQUARE-ROOT 2 X SQUARE-ROOT 3)R30-DEGREES-S ADSORBATE STRUCTURE [J].
MACA, F ;
SCHEFFLER, M ;
BERNDT, W .
SURFACE SCIENCE, 1985, 160 (02) :467-474
[10]   INTERACTION OF THE PT(111) SURFACE WITH ADSORBED XE ATOMS [J].
MULLER, JE .
PHYSICAL REVIEW LETTERS, 1990, 65 (24) :3021-3024