ENHANCED NONLINEAR-OPTICAL RESPONSE OF COMPOSITE-MATERIALS

被引:175
作者
FISCHER, GL
BOYD, RW
GEHR, RJ
JENEKHE, SA
OSAHENI, JA
SIPE, JE
WELLERBROPHY, LA
机构
[1] UNIV ROCHESTER,INST OPT,ROCHESTER,NY 14627
[2] UNIV ROCHESTER,DEPT CHEM ENGN,ROCHESTER,NY 14627
[3] UNIV TORONTO,DEPT PHYS,TORONTO,ON M5S 1A7,CANADA
[4] THREE M CO,DIV TELECOM SYST,AUSTIN,TX 78726
关键词
D O I
10.1103/PhysRevLett.74.1871
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We present experimental results which demonstrate that the effective third-order susceptibility of a composite optical material can exceed those of the materials from which it is constructed. In particular, we have formed a composite of alternating, sub-wavelength-thick layers of titanium dioxide and the conjugated polymer poly (p-phenylene-benzobisthiazole), and find that its nonlinear susceptibility exceeds that of its more nonlinear constituent by 35%. The enhancement of the nonlinear susceptibility, which under more ideal but still realistic conditions can be as large as a factor of 10, can be understood as a consequence of local field corrections. © 1995 The American Physical Society.
引用
收藏
页码:1871 / 1874
页数:4
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