THE TROPOSPHERIC DISTRIBUTION OF FORMALDEHYDE DURING TROPOZ-II

被引:59
作者
ARLANDER, DW [1 ]
BRUNING, D [1 ]
SCHMIDT, U [1 ]
EHHALT, DH [1 ]
机构
[1] FORSCHUNGSZENTRUM JULICH, FORSCHUNGSZENTRUM, INST ATMOSPHAR CHEM, D-52425 JULICH, GERMANY
关键词
FORMALDEHYDE; BACKGROUND TROPOSPHERE; CONCENTRATION DISTRIBUTION; AIRCRAFT; SAMPLING TECHNIQUE; METHANE OXIDATION;
D O I
10.1007/BF00696637
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
A series of 149 measurements of the HCHO mixing ratio were made between 0 and 10 km altitude and 70 degrees N to 60 degrees S latitude during TROPOZ II. The data show a vertical decrease of the HCHO mixing ratio with altitude at all latitudes and a broad latitudinal maximum in the HCHO mixing ratio between 30 degrees N and 30 degrees S at all altitudes. The measured mixing ratios of HCHO are considerably higher than those expected from CH4 oxidation alone, but agree broadly with the average latitude by altitude distribution of HCHO derived by a 2D model including emissions of C-1-C-7 hydrocarbons. A number of the regional scale deviations of the measured HCHO distribution from the average modelled one can be explained in terms of the local wind field.
引用
收藏
页码:251 / 269
页数:19
相关论文
共 13 条
[1]   GASEOUS OXYGENATED HYDROCARBONS IN THE REMOTE MARINE TROPOSPHERE [J].
ARLANDER, DW ;
CRONN, DR ;
FARMER, JC ;
MENZIA, FA ;
WESTBERG, HH .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1990, 95 (D10) :16391-16403
[2]  
ARLANDER DW, 1995, J ATMOS CHEM, V22, P241
[3]  
ARLANDER DW, 1992, 2650 U KOLN FORSCH J
[4]   GAS-PHASE TROPOSPHERIC CHEMISTRY OF ORGANIC-COMPOUNDS - A REVIEW [J].
ATKINSON, R .
ATMOSPHERIC ENVIRONMENT PART A-GENERAL TOPICS, 1990, 24 (01) :1-41
[5]   SAMPLING OF FORMALDEHYDE IN AIR WITH COATED SOLID SORBENT AND DETERMINATION BY HIGH-PERFORMANCE LIQUID-CHROMATOGRAPHY [J].
BEASLEY, RK ;
HOFFMANN, CE ;
RUEPPEL, ML ;
WORLEY, JW .
ANALYTICAL CHEMISTRY, 1980, 52 (07) :1110-1114
[6]   A NEW TECHNIQUE FOR COLLECTION, CONCENTRATION AND DETERMINATION OF GASEOUS TROPOSPHERIC FORMALDEHYDE [J].
COFER, WR ;
EDAHL, RA .
ATMOSPHERIC ENVIRONMENT, 1986, 20 (05) :979-984
[8]   A NEW TECHNIQUE FOR MEASURING TROPOSPHERIC FORMALDEHYDE [CH2O] [J].
LOWE, DC ;
SCHMIDT, U ;
EHHALT, DH .
GEOPHYSICAL RESEARCH LETTERS, 1980, 7 (10) :825-828
[9]   MERIDIONAL AND VERTICAL CO AND CH4 DISTRIBUTIONS IN THE BACKGROUND TROPOSPHERE (70-DEGREES-N-60-DEGREES-S - 0-12KM ALTITUDE) FROM SCIENTIFIC AIRCRAFT MEASUREMENTS DURING THE STRATOZ-III EXPERIMENT (JUNE 1984) [J].
MARENCO, A ;
MACAIGNE, M ;
PRIEUR, S .
ATMOSPHERIC ENVIRONMENT, 1989, 23 (01) :185-200
[10]   GLOBAL AVERAGE CONCENTRATION AND TREND FOR HYDROXYL RADICALS DEDUCED FROM ALE GAUGE TRICHLOROETHANE (METHYL CHLOROFORM) DATA FOR 1978-1990 [J].
PRINN, R ;
CUNNOLD, D ;
SIMMONDS, P ;
ALYEA, F ;
BOLDI, R ;
CRAWFORD, A ;
FRASER, P ;
GUTZLER, D ;
HARTLEY, D ;
ROSEN, R ;
RASMUSSEN, R .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1992, 97 (D2) :2445-2461