INFRARED PUMP-PROBE SPECTROSCOPY OF WATER AT SUBPICOSECOND TIME SCALES - A THEORY

被引：9

作者：

BRATOS, S

LEICKNAM, JC

机构：

[1] Laboratoire de Physique Théorique, Liquides Université Pierre et Marie Curie, 75252 Paris Cedex 05, Case courrier 121

来源：

JOURNAL OF MOLECULAR LIQUIDS | 1995年 / 64卷 / 1-2期

关键词：

D O I：

10.1016/0167-7322(95)92827-X

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

A theory is presented to describe pump-probe infrared spectra of water at subpicosecond time scales, comparable to those characteristic of spectral diffusion. This theory is a statistical theory using a correlation function description of the nonlinear optical processes involved. It predicts real time shifts of spectral bands, preceded by a redistribution of their intensities. Physical interpretation of these findings is proposed.

引用

页码：151 / 159

页数：9

共 16 条

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