NO STICKING ON A PT(111) SURFACE

被引:32
作者
BROWN, JK [1 ]
LUNTZ, AC [1 ]
机构
[1] IBM RES,ALMADEN RES CTR,SAN JOSE,CA 95120
关键词
D O I
10.1016/0009-2614(93)89185-K
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The dependence of the initial sticking coefficient of NO on a Pt(111) surface has been measured as a function of initial energy and angle by molecular beam techniques. This shows a gradual decrease with increasing energy over the entire accessible energy range of 3 eV. No dissociation was observable for incident energies up to 1.5 eV. These results are shown by stochastic trajectory calculations to be qualitatively compatible with a reasonable NO-Pt(111) interaction potential.
引用
收藏
页码:451 / 454
页数:4
相关论文
共 13 条
[1]   VIBRATIONAL AND ROTATIONAL ENERGY-DISTRIBUTION OF NO SCATTERED FROM THE PT(111) CRYSTAL-SURFACE - DETECTION BY 2-PHOTON IONIZATION [J].
ASSCHER, M ;
GUTHRIE, WL ;
LIN, TH ;
SOMORJAI, GA .
PHYSICAL REVIEW LETTERS, 1982, 49 (01) :76-79
[2]   A MOLECULAR-BEAM STUDY ON THE INTERACTION OF NO WITH A PT(111) SURFACE [J].
CAMPBELL, CT ;
ERTL, G ;
SEGNER, J .
SURFACE SCIENCE, 1982, 115 (02) :309-322
[3]   ROTATIONALLY INELASTIC GAS-SURFACE SCATTERING INVESTIGATED BY LASER-INDUCED FLUORESCENCE [J].
FRENKEL, F ;
HAGER, J ;
KRIEGER, W ;
WALTHER, H ;
CAMPBELL, CT ;
ERTL, G ;
KUIPERS, H ;
SEGNER, J .
PHYSICAL REVIEW LETTERS, 1981, 46 (02) :152-155
[4]   NITRIC-OXIDE ADSORPTION ON THE PT(111) SURFACE [J].
GLAND, JL ;
SEXTON, BA .
SURFACE SCIENCE, 1980, 94 (2-3) :355-368
[5]   STICKING AND SCATTERING IN THE MOLECULAR CHEMISORPTION REGIME - CO ON PT(111) [J].
HARRIS, J ;
LUNTZ, AC .
JOURNAL OF CHEMICAL PHYSICS, 1989, 91 (10) :6421-6428
[6]   ROTATIONAL ALIGNMENT OF NO DESORBING FROM PT(111) [J].
JACOBS, DC ;
KOLASINSKI, KW ;
MADIX, RJ ;
ZARE, RN .
JOURNAL OF CHEMICAL PHYSICS, 1987, 87 (08) :5038-5039
[7]   SIMPLIFIED TRAJECTORY METHOD FOR MODELING GAS SURFACE SCATTERING - THE NO/PT(111) SYSTEM [J].
JACOBS, DC ;
ZARE, RN .
JOURNAL OF CHEMICAL PHYSICS, 1989, 91 (05) :3196-3207
[8]   ROTATIONAL POPULATION AND ALIGNMENT DISTRIBUTIONS FOR INELASTIC-SCATTERING AND TRAPPING DESORPTION OF NO ON PT(111) [J].
JACOBS, DC ;
KOLASINSKI, KW ;
SHANE, SF ;
ZARE, RN .
JOURNAL OF CHEMICAL PHYSICS, 1989, 91 (05) :3182-3195
[9]   REACTION-MECHANISM IN CHEMISORPTION KINETICS - NITROGEN ON (100) PLANE OF TUNGSTEN [J].
KING, DA ;
WELLS, MG .
PROCEEDINGS OF THE ROYAL SOCIETY OF LONDON SERIES A-MATHEMATICAL AND PHYSICAL SCIENCES, 1974, 339 (1617) :245-269
[10]   STERIC EFFECTS FOR NO/PT(111) ADSORPTION AND SCATTERING [J].
KUIPERS, EW ;
TENNER, MG ;
KLEYN, AW ;
STOLTE, S .
PHYSICAL REVIEW LETTERS, 1989, 62 (18) :2152-2155