A CLOSE-COUPLING STUDY OF COLLISION-INDUCED DISSOCIATION IN HE+H-2

被引:16
作者
NOBUSADA, K [1 ]
SAKIMOTO, K [1 ]
ONDA, K [1 ]
机构
[1] SCI UNIV TOKYO,FAC IND SCI & TECHNOL,OSHAMANBE,HOKKAIDO 04935,JAPAN
关键词
D O I
10.1016/0009-2614(94)01462-5
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The previous quantum mechanical close-coupling study of the dissociative collisions in He+H-2 (T-shape configuration) by the present authors [Chem. Phys. Letters 216 (1993) 613] has been extended to a wide range of the total energy 4.8-7.5 eV. The dissociation process shows a clear vibrational enhancement. The dissociation probability has an undulation as a function of the total energy, and by using classical S-matrix theory it is shown that this feature is caused by interference of the contributions of multiple trajectories.
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页码:399 / 404
页数:6
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