NUCLEAR-REACTION ANALYSIS OF DEUTERIUM DIFFUSION IN ZR-2.5 WT-PERCENT NB PRESSURE TUBE MATERIAL

被引:9
作者
LAURSEN, T [1 ]
LEGER, M [1 ]
WHITTON, JL [1 ]
机构
[1] ONTARIO HYDRO,TORONTO M8Z 5S4,ONTARIO,CANADA
关键词
Nuclear Reactors--Materials - Tubes - Zirconium Niobium Alloys--Analysis;
D O I
10.1016/0022-3115(88)90153-5
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Nuclear reaction analysis (NRA) has been used to measure the diffusion coefficient of deuterium in Zr-2.5 wt percent Nb pressure tube material. The measured diffusion coefficient is 1.13×10-10 m2 s-1 at 300°C and 1.23×10-10 m2 s-1 at 350°C. The results are in reasonable agreement with measurements carried out by vacuum extraction analysis. The value obtained for the diffusion coefficient at 350°C is lower than a prediction based on measurements at lower temperatures and may be showing the influence of the break-up of the β-phase, although some effect due to tube-to-tube variability cannot be discounted. NRA detects a surface deuterium peak which is shown to correlate with the bulk deuteride concentration.
引用
收藏
页码:49 / 56
页数:8
相关论文
共 8 条
[1]   CANDU-PHW PRESSURE TUBES - THEIR MANUFACTURE, INSPECTION, AND PROPERTIES [J].
CHEADLE, BA ;
COLEMAN, CE ;
LICHT, H .
NUCLEAR TECHNOLOGY, 1982, 57 (03) :413-425
[2]   ANALYSIS AND DEPTH PROFILING OF DEUTERIUM WITH THE DCHE-3,P)HE-4 REACTION BY DETECTING THE PROTONS AT BACKWARD ANGLES [J].
DIEUMEGARD, D ;
DUBREUIL, D ;
AMSEL, G .
NUCLEAR INSTRUMENTS & METHODS, 1979, 166 (03) :431-445
[3]   NUCLEAR-REACTION ANALYSIS OF DEUTERIUM IN DEUTERIDED ZR-2.5 WT-PERCENT NB ALLOY [J].
LAURSEN, T ;
KOELBL, RS .
JOURNAL OF NUCLEAR MATERIALS, 1986, 137 (03) :241-249
[4]  
Leger M., 1980, 80223K ONT HYDR RES
[5]  
LEGER M, 1982, M82155K ONT HYDR RES
[6]  
Northwood D. O., 1983, International Metals Reviews, V28, P92
[7]  
SAWATZKY A, 1981, AECL7265 AT EN CAN R
[8]   HYDROGEN AND DEUTERIUM PROFILING AT THE SURFACE OF ZIRCONIUM ALLOYS .1. THE EFFECTS OF SURFACE PREPARATION [J].
STERN, A ;
KHATAMIAN, D ;
LAURSEN, T ;
WEATHERLY, GC ;
PERZ, JM .
JOURNAL OF NUCLEAR MATERIALS, 1987, 144 (1-2) :35-42