Evasion of mercury vapor from tee surface of a recently limed acid forest lake in Sweden

被引:41
作者
Lindberg, SE
Meyers, TP
Munthe, J
机构
[1] OAK RIDGE NATL LAB,DIV ENVIRONM SCI,OAK RIDGE,TN 37831
[2] NOAA,ATMOSPHER TURBULENCE & DIFFUS DIV,OAK RIDGE,TN
关键词
D O I
10.1007/BF00476915
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Mercury is emitted from soil and water surfaces, but few actual direct flux measurements have been reported. During June, 1994 we performed the first micrometeorological measurements of Hg vapor fluxes over a boreal forest lake. Using highly precise methods with multiple replicate samplers, we measured concentration gradients of Hg vapor, CO2 and H2O over the lake surface. Mercury was readily emitted from the lake surface, and we found no evidence of Hg dry deposition to the lake. Emission rates over the lake averaged 8.5 ng m(-2) h(-1), and appeared to be weakly influenced by water temperature and solar radiation. These fluxes were somewhat higher than those previously measured using surface chambers at this site.
引用
收藏
页码:725 / 730
页数:6
相关论文
共 13 条
[1]   SUNLIGHT-INDUCED FORMATION OF DISSOLVED GASEOUS MERCURY IN LAKE WATERS [J].
AMYOT, M ;
MIERLE, G ;
LEAN, DRS ;
MCQUEEN, DJ .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1994, 28 (13) :2366-2371
[2]   MEASURING BIOSPHERE-ATMOSPHERE EXCHANGES OF BIOLOGICALLY RELATED GASES WITH MICROMETEOROLOGICAL METHODS [J].
BALDOCCHI, DD ;
HICKS, BB ;
MEYERS, TP .
ECOLOGY, 1988, 69 (05) :1331-1340
[3]   DETERMINATION OF VOLATILE MERCURY SPECIES AT THE PICOGRAM LEVEL BY LOW-TEMPERATURE GAS-CHROMATOGRAPHY WITH COLD-VAPOR ATOMIC FLUORESCENCE DETECTION [J].
BLOOM, N ;
FITZGERALD, WF .
ANALYTICA CHIMICA ACTA, 1988, 208 (1-2) :151-161
[4]  
Fitzgerald W. F., 1994, P203
[5]   MERCURY IN FOREST CANOPY THROUGHFALL WATER AND ITS RELATION TO ATMOSPHERIC DEPOSITION [J].
IVERFELDT, A .
WATER AIR AND SOIL POLLUTION, 1991, 56 :553-564
[6]   MICROMETEOROLOGICAL MEASUREMENTS OF MERCURY-VAPOR FLUXES OVER BACKGROUND FOREST SOILS IN EASTERN TENNESSEE [J].
KIM, KH ;
LINDBERG, SE ;
MEYERS, TP .
ATMOSPHERIC ENVIRONMENT, 1995, 29 (02) :267-282
[7]   High-precision measurements of mercury vapor in air: Design of a six-port-manifold mass flow controller system and evaluation of mass flow errors at atmospheric pressure [J].
Kim, Ki-Hyun ;
Lindberg, Steven E. .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1994, 99 (D3) :5379-5384
[8]   MICROMETEOROLOGICAL GRADIENT APPROACH FOR QUANTIFYING AIR-SURFACE EXCHANGE OF MERCURY-VAPOR - TESTS OVER CONTAMINATED SOILS [J].
LINDBERG, SE ;
KIM, KH ;
MEYERS, TP ;
OWENS, JG .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1995, 29 (01) :126-135
[9]   ATMOSPHERIC EMISSION AND PLANT UPTAKE OF MERCURY FROM AGRICULTURAL SOILS NEAR THE ALMADEN MERCURY MINE [J].
LINDBERG, SE ;
JACKSON, DR ;
HUCKABEE, JW ;
JANZEN, SA ;
LEVIN, MJ ;
LUND, JR .
JOURNAL OF ENVIRONMENTAL QUALITY, 1979, 8 (04) :572-578
[10]  
MEYERS TP, 1993, J GEOPHYS RES, V7, P7