DOUBLE-RESONANT 2ND HARMONIC-GENERATION FROM SURFACE COVERAGES OF NILE-BLUE-A

被引:33
作者
MAROWSKY, G
GIERULSKI, A
DICK, B
机构
[1] Max-Planck-Inst fuer, Biophysikalische Chemie, Goettingen,, West Ger, Max-Planck-Inst fuer Biophysikalische Chemie, Goettingen, West Ger
关键词
HARMONIC GENERATION;
D O I
10.1016/0030-4018(85)90197-X
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Second harmonic emission from a dye covered quartz surface has been observed in total internal reflection. Coverages with the dye nile-blue A yielded an increase in second harmonic output by several orders of magnitude as compared to coverages with rhodamine 6G. In the latter case only the harmonic light is at resonance with the S//0-S//2 transition of the adsorbed dye molecules, whereas for nile-blue A both, the fundamental and the harmonic frequency, are at resonance with the respective singlet transitions.
引用
收藏
页码:339 / 342
页数:4
相关论文
共 14 条
[1]   LIGHT WAVES AT BOUNDARY OF NONLINEAR MEDIA [J].
BLOEMBERGEN, N ;
PERSHAN, PS .
PHYSICAL REVIEW, 1962, 128 (02) :606-+
[2]  
Bloembergen N., 1977, NONLINEAR OPTICS
[3]   SURFACE-ENCHANCED 2ND-HARMONIC GENERATION [J].
CHEN, CK ;
DECASTRO, ARB ;
SHEN, YR .
PHYSICAL REVIEW LETTERS, 1981, 46 (02) :145-148
[4]   DETECTION OF MOLECULAR MONOLAYERS BY OPTICAL 2ND-HARMONIC GENERATION [J].
CHEN, CK ;
HEINZ, TF ;
RICARD, D ;
SHEN, YR .
PHYSICAL REVIEW LETTERS, 1981, 46 (15) :1010-1012
[5]   SPECTROSCOPIC AND LINE-NARROWING PROPERTIES OF RESONANT SUM AND DIFFERENCE FREQUENCY GENERATION [J].
DICK, B ;
HOCHSTRASSER, RM .
JOURNAL OF CHEMICAL PHYSICS, 1983, 78 (06) :3398-3409
[6]  
DICK B, UNPUB
[7]  
HEINZ TF, 1982, PHYS REV LETT, V48, P478, DOI 10.1103/PhysRevLett.48.478
[8]   DETERMINATION OF MOLECULAR-ORIENTATION OF MONOLAYER ADSORBATES BY OPTICAL 2ND-HARMONIC GENERATION [J].
HEINZ, TF ;
TOM, HWK ;
SHEN, YR .
PHYSICAL REVIEW A, 1983, 28 (03) :1883-1885
[9]  
HEINZ TF, 1984, 13 IQEC AN
[10]   EFFECTS OF DISPERSION AND FOCUSING ON PRODUCTION OF OPTICAL HARMONICS [J].
MAKER, PD ;
SAVAGE, CM ;
TERHUNE, RW ;
NISENOFF, M .
PHYSICAL REVIEW LETTERS, 1962, 8 (01) :21-&