PHOTON ANTIBUNCHING IN THE FLUORESCENCE OF A SINGLE DYE MOLECULE TRAPPED IN A SOLID

被引:492
作者
BASCHE, T
MOERNER, WE
ORRIT, M
TALON, H
机构
[1] CNRS, CTR PHYS MOLEC OPT & HERTZIENNE, F-33405 TALENCE, FRANCE
[2] UNIV BORDEAUX 1, F-33405 TALENCE, FRANCE
关键词
D O I
10.1103/PhysRevLett.69.1516
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The correlation between fluorescence photons emitted by an optically pumped single molecule of pentacene in a p-terphenyl host has been investigated at short times. The correlation function shows photon antibunching, a unique feature of a nonclassical radiation field, which decreases if two molecules rather than one are pumped at the same time. The peculiarities of the correlation function for a three-level molecule are discussed and the theoretical description outlined.
引用
收藏
页码:1516 / 1519
页数:4
相关论文
共 20 条
[1]   FLUORESCENCE SPECTROSCOPY AND SPECTRAL DIFFUSION OF SINGLE IMPURITY MOLECULES IN A CRYSTAL [J].
AMBROSE, WP ;
MOERNER, WE .
NATURE, 1991, 349 (6306) :225-227
[2]   DETECTION AND SPECTROSCOPY OF SINGLE PENTACENE MOLECULES IN A PARA-TERPHENYL CRYSTAL BY MEANS OF FLUORESCENCE EXCITATION [J].
AMBROSE, WP ;
BASCHE, T ;
MOERNER, WE .
JOURNAL OF CHEMICAL PHYSICS, 1991, 95 (10) :7150-7163
[3]   OPTICAL MODIFICATION OF A SINGLE IMPURITY MOLECULE IN A SOLID [J].
BASCHE, T ;
MOERNER, WE .
NATURE, 1992, 355 (6358) :335-337
[4]   PROPOSAL FOR MEASUREMENT OF RESONANT STARK EFFECT BY PHOTON CORRELATION TECHNIQUES [J].
CARMICHAEL, HJ ;
WALLS, DF .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 1976, 9 (04) :L43-L46
[5]  
DEHMELT HG, 1983, ADV LASER SPECTROSCO
[6]   LASER EXPERIMENTS WITH SINGLE ATOMS AS A TEST OF BASIC PHYSICS [J].
DIEDRICH, F ;
KRAUSE, J ;
REMPE, G ;
SCULLY, MO ;
WALTHER, H .
IEEE JOURNAL OF QUANTUM ELECTRONICS, 1988, 24 (07) :1314-1319
[7]   NONCLASSICAL RADIATION OF A SINGLE STORED ION [J].
DIEDRICH, F ;
WALTHER, H .
PHYSICAL REVIEW LETTERS, 1987, 58 (03) :203-206
[8]   LASER SPECTROSCOPY OF TRAPPED ATOMIC IONS [J].
ITANO, WM ;
BERGQUIST, JC ;
WINELAND, DJ .
SCIENCE, 1987, 237 (4815) :612-617
[9]   MULTIATOM AND TRANSIT-TIME EFFECTS ON PHOTON-CORRELATION MEASUREMENTS IN RESONANCE FLUORESCENCE [J].
KIMBLE, HJ ;
DAGENAIS, M ;
MANDEL, L .
PHYSICAL REVIEW A, 1978, 18 (01) :201-207
[10]   PHOTON ANTI-BUNCHING IN RESONANCE FLUORESCENCE [J].
KIMBLE, HJ ;
DAGENAIS, M ;
MANDEL, L .
PHYSICAL REVIEW LETTERS, 1977, 39 (11) :691-695