LOW-TEMPERATURE DYNAMICS IN GLASSES AND THE STOCHASTIC SUDDEN-JUMP MODEL

被引:51
作者
SUAREZ, A [1 ]
SILBEY, R [1 ]
机构
[1] MIT,DEPT CHEM,CAMBRIDGE,MA 02139
关键词
D O I
10.1016/0009-2614(94)00033-6
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Non-linear optical experiments in glasses exhibiting spectral diffusion give strong support for the importance of two-level system excitations (TLS). The difference in the line widths measured by these experiments and fast two-pulse photon echo experiments has been ascribed to slowly relaxing TLS. The sudden jump model is found to be an appropriate description of the dynamics; within this model, we derive new analytical results for three-pulse experiments at all temperatures. These experiments and the dynamics of TLS in glasses are discussed within the context of these results.
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页码:445 / 453
页数:9
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