THE PULSED-ARC CLUSTER ION-SOURCE (PACIS)

被引:105
作者
SIEKMANN, HR
LUDER, C
FAEHRMANN, J
LUTZ, HO
MEIWESBROER, KH
机构
[1] Fakultät für Physik, Universität Bielefeld, Bielefeld 1
来源
ZEITSCHRIFT FUR PHYSIK D-ATOMS MOLECULES AND CLUSTERS | 1991年 / 20卷 / 1-4期
关键词
D O I
10.1007/BF01544026
中图分类号
O64 [物理化学(理论化学)、化学物理学]; O56 [分子物理学、原子物理学];
学科分类号
070203 ; 070304 ; 081704 ; 1406 ;
摘要
A new cluster source, the "PACIS", has recently been developed [1, 2]: a pulsed high-current arc is fired between two electrically isolated electrodes. In a stream of carrier gas, the nascent metal plasma cools down, thus undergoes significant aggregation. After supersonic expansion into high vacuum, the resulting cluster ions will be subject to investigation. Here, we present the current state of the source development and further technical details. The integral intensity is estimated by film thickness measurements and yields a deposition rate of, e.g., up to 2 angstrom per shot for lead. About 10% of the emitted material turns out to be charged. Time-of-flight measurements show similar cluster ion mass spectra as they are known from laser vaporization. Already single shot mass spectra display complete n-series which can be followed to n almost-equal-to 40. For heavy clusters, a significant velocity slip is estimated from the beam velocities.
引用
收藏
页码:417 / 420
页数:4
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