ATMOSPHERIC METHANE - RECENT GLOBAL TRENDS

被引:105
作者
KHALIL, MAK
RASMUSSEN, RA
机构
[1] Institute of Atmospheric Sciences, Oregon Graduate Center, Beaverton
关键词
Hydrocarbons--Concentration - Methane--Environmental Testing;
D O I
10.1021/es00074a014
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
We report globally averaged concentrations of atmospheric methane for every month of the past 8 years based on measurements taken at six locations ranging in latitude from within the Arctic Circle to the South Pole. This record shows that methane concentration increased at an average rate of 16.6 ± 0.4 ppbv/yr or ~1.02 ± 0.02%/yr over 8 years. This trend has not been constant according to our record but has varied between 12 ± 2 and 23 ± 2 ppbv/yr over 2-year periods after seasonal variations are removed. The causes of these interannual variations are not known. We also show that the total mass of methane in the earth's atmosphere undergoes seasonal variations, with highest levels during late fall and early winters of the northern hemisphere and lowest levels in the summers. After the main features of the record are taken into account, residual random fluctuations remain, which have a variability of only 3 ppbv or 0.2% of the mean concentrations. The variation of the trends at different times during the past decade accounts for the differences of trends reported in various studies. Uncertainties in our estimates are reported as 90% confidence limits. © 1990, American Chemical Society. All rights reserved.
引用
收藏
页码:549 / 553
页数:5
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