GENERATION AND PHOTOIONIZATION OF COLD NAN CLUSTERS - N TO 200

被引：60

作者：

HONEA, EC ^{[1
]}

HOMER, ML ^{[1
]}

PERSSON, JL ^{[1
]}

WHETTEN, RL ^{[1
]}

机构：

[1] UNIV CALIF LOS ANGELES,DEPT PHYS,LOS ANGELES,CA 90024

来源：

CHEMICAL PHYSICS LETTERS | 1990年 / 171卷 / 03期

关键词：

D O I：

10.1016/0009-2614(90)85218-2

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Featureless abundance distributions are found for sodium atomic clusters in a cold He flowstream by laser ablation, demonstrating that the "magic number" ledges observed previously from oven-beam experiments are caused by high cluster temperatures. The utility of the cold pulsed beams indicated here by experiments on photoionization and photofragmentation properties, including ionization potential estimates for n as large as 137. Electronic and chemical measurements on cold alkali metal clusters in beams or flowing gases will permit critical tests of the electronic shell model. © 1990.

引用

页码：147 / 154

页数：8

共 48 条

[1]

ALVAREZ MM, UNPUB MASSYIELDS LAS

[2]

Andreoni W., 1988, Elemental and Molecular Clusters. Proceedings of the 13th International School, P206

[3] TEMPERATURE AND SEGREGATION EFFECTS IN ALKALI-METAL MICROCLUSTERS FROM ABINITIO MOLECULAR-DYNAMICS SIMULATIONS [J].