WAVE-PACKET STRUCTURE AND DYNAMICS MEASURED BY COULOMB EXPLOSION

被引:147
作者
STAPELFELDT, H [1 ]
CONSTANT, E [1 ]
CORKUM, PB [1 ]
机构
[1] UNIV SHERBROOKE,FAC SCI,DEPT PHYS,SHERBROOKE,PQ J1K 2R1,CANADA
关键词
D O I
10.1103/PhysRevLett.74.3780
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The motion and dimension of molecular nuclear wave packets produced by an ultrashort laser pulse are measured by Coulomb explosion induced by a delayed intense fs laser pulse. Two different continuum wave packets in I2 are observed as they move from an internuclear separation of ∼7 to >100 Å. The ultimate spatial resolution is limited by the pulse duration of the probe laser. For 485 nm excitation of B-state wave packets the resolution limit is ∼0.5 Å. © 1995 The American Physical Society.
引用
收藏
页码:3780 / 3783
页数:4
相关论文
共 18 条
[1]   FEMTOSECOND PROBING OF SODIUM CLUSTER ION NAN + FRAGMENTATION [J].
BAUMERT, T ;
ROTTGERMANN, C ;
ROTHENFUSSER, C ;
THALWEISER, R ;
WEISS, V ;
GERBER, G .
PHYSICAL REVIEW LETTERS, 1992, 69 (10) :1512-1515
[2]   TRANSIENT-X-RAY SCATTERING CALCULATED FROM MOLECULAR-DYNAMICS [J].
BERGSMA, JP ;
COLADONATO, MH ;
EDELSTEN, PM ;
KAHN, JD ;
WILSON, KR ;
FREDKIN, DR .
JOURNAL OF CHEMICAL PHYSICS, 1986, 84 (11) :6151-6160
[3]   MOLECULAR-REORIENTATION DURING DISSOCIATIVE MULTIPHOTON IONIZATION [J].
DIETRICH, P ;
STRICKLAND, DT ;
LABERGE, M ;
CORKUM, PB .
PHYSICAL REVIEW A, 1993, 47 (03) :2305-2311
[4]   EXPERIMENTAL-DETERMINATION OF THE DYNAMICS OF A MOLECULAR NUCLEAR WAVE-PACKET VIA THE SPECTRA OF SPONTANEOUS EMISSION [J].
DUNN, TJ ;
SWEETSER, JN ;
WALMSLEY, IA ;
RADZEWICZ, C .
PHYSICAL REVIEW LETTERS, 1993, 70 (22) :3388-3391
[5]  
FISCHER I, IN PRESS J CHEM PHYS
[6]   PHOTOIONIZATION AND FRAGMENTATION DYNAMICS OF C-60 [J].
HOHMANN, H ;
CALLEGARI, C ;
FURRER, S ;
GROSENICK, D ;
CAMPBELL, EEB ;
HERTEL, IV .
PHYSICAL REVIEW LETTERS, 1994, 73 (14) :1919-1922
[7]  
IVANOV MY, UNPUB
[8]   TIME-RESOLVED LUMINESCENCE FROM COHERENTLY EXCITED MOLECULES AS A PROBE OF MOLECULAR WAVE-PACKET DYNAMICS [J].
KOWALCZYK, P ;
RADZEWICZ, C ;
MOSTOWSKI, J ;
WALMSLEY, IA .
PHYSICAL REVIEW A, 1990, 42 (09) :5622-5626
[9]   OPTICAL CONTROL OF MOLECULAR-DYNAMICS - MOLECULAR CANNONS, REFLECTRONS, AND WAVE-PACKET FOCUSERS [J].
KRAUSE, JL ;
WHITNELL, RM ;
WILSON, KR ;
YAN, YJ ;
MUKAMEL, S .
JOURNAL OF CHEMICAL PHYSICS, 1993, 99 (09) :6562-6578