DECAY CHANNELS OF CORE-EXCITED H2S STUDIED BY SYNCHROTRON-RADIATION-EXCITED PHOTOELECTRON-SPECTROSCOPY

被引:43
作者
AKSELA, H
AKSELA, S
DEBRITO, AN
BANCROFT, GM
TAN, KH
机构
[1] UNIV WESTERN ONTARIO, DEPT CHEM, LONDON N6A 5B7, ONTARIO, CANADA
[2] UNIV WESTERN ONTARIO, CTR CHEM PHYS, LONDON N6A 5B7, ONTARIO, CANADA
[3] UNIV WISCONSIN, CTR SYNCHROTRON RADIAT, CANADIAN SYNCHROTRON RADIAT FACIL, STOUGHTON, WI 53589 USA
来源
PHYSICAL REVIEW A | 1992年 / 45卷 / 11期
关键词
D O I
10.1103/PhysRevA.45.7948
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
The 2p(3a,) to 6a, and 3b2 photoexcitation resonance of H2S has been studied using synchrotron-radiation-excited photoelectron spectroscopy. The overall shape of the measured photoelectron spectrum of H2S is found to be in close resemblance with the normal Auger-electron spectrum of HCl. The spectrum is assumed to result mainly from the Auger decay in the excited HS molecule taking place after the molecular dissociation of the excited H2S Molecule. The finding is compared with the results of multiconfiguration self-consistent-field calculations
引用
收藏
页码:7948 / 7952
页数:5
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