HYDRODYNAMICS AND MASS TRANSFER IN DOWNFLOW BUBBLE COLUMN

被引:23
作者
Kulkarni, Amol [1 ]
Shah, Yatish [1 ]
Schumpe, Adrian [1 ]
机构
[1] Univ Pittsburgh, Dept Chem & Petr Engn, Pittsburgh, PA 15261 USA
关键词
D O I
10.1080/00986448308940089
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Gas holdup, effective interfacial area and volumetric mass transfer coefficient were measured in two and three phase downflow bubble columns. The mass transfer data were obtained using the chemical method of sulfite oxidation. and the gas holdup was measured using the hydrostatic technique. Glass beads and Triton 114 were used to study the effects of solids and liquid surface tension on the gas holdup and the mass transfer parameters g and k(L)(a) under bar. The gas holdup in three phase systems was measured for non-wettable (glass bead) and wettable (coal and shale particles) solids. The mass transfer data obtained in the down flow bubble column were compared with the values published for up flow bubble columns. The results indicate that in the range of superficial gas velocities (0.002-0.025) m/s investigated, the values of the mass transfer coefficient were of the same order of magnitude as those observed in upflow systems, but the values of interfacial area were at least two fold greater. Also, the results showed that the operating variables and the physical properties had different influences on (a) under bar and k(L)(a) under bar in the downflow bubble column. Correlations for (a) under bar and k(L)(a) under bar for the downflow bubble column are proposed which predict the data with adequate accuracy in the range of operating conditions investigated.
引用
收藏
页码:307 / 337
页数:31
相关论文
共 41 条
[1]   BUBBLE SIZE, INTERFACIAL AREA, AND LIQUID-PHASE MASS-TRANSFER COEFFICIENT IN BUBBLE COLUMNS [J].
AKITA, K ;
YOSHIDA, F .
INDUSTRIAL & ENGINEERING CHEMISTRY PROCESS DESIGN AND DEVELOPMENT, 1974, 13 (01) :84-91
[2]   GAS HOLDUP AND VOLUMETRIC MASS-TRANSFER COEFFICIENT IN BUBBLE COLUMNS - EFFECTS OF LIQUID PROPERTIES [J].
AKITA, K ;
YOSHIDA, F .
INDUSTRIAL & ENGINEERING CHEMISTRY PROCESS DESIGN AND DEVELOPMENT, 1973, 12 (01) :76-80
[3]  
ARMSTRONG ER, 1976, FLUIDIZATION TECHNOL
[4]   EFFECT OF SOLIDS WETTABILITY ON EXPANSION OF GAS-LIQUID FLUIDIZED-BEDS [J].
BHATIA, VK ;
EVANS, KA ;
EPSTEIN, N .
INDUSTRIAL & ENGINEERING CHEMISTRY PROCESS DESIGN AND DEVELOPMENT, 1972, 11 (01) :151-&
[5]  
Calderbank P.H, 1967, CHEM ENG-NEW YORK, V45, P209
[6]   THE CONTINUOUS PHASE HEAT AND MASS-TRANSFER PROPERTIES OF DISPERSIONS [J].
CALDERBANK, PH ;
MOOYOUNG, MB .
CHEMICAL ENGINEERING SCIENCE, 1961, 16 (1-2) :39-54
[7]  
CARLETON AJ, 1977, CHEM ENG SCI, V32, P1427
[8]   HYDRODYNAMIC PROPERTIES OF THE FISCHER-TROPSCH SLURRY PROCESS [J].
DECKWER, WD ;
LOUISI, Y ;
ZAIDI, A ;
RALEK, M .
INDUSTRIAL & ENGINEERING CHEMISTRY PROCESS DESIGN AND DEVELOPMENT, 1980, 19 (04) :699-708
[9]   FLOW AND OXYGEN-TRANSFER IN COCURRENT GAS-LIQUID DOWNFLOW [J].
FUJIE, K ;
TAKAINE, M ;
KUBOTA, H ;
MIYAJI, Y .
JOURNAL OF CHEMICAL ENGINEERING OF JAPAN, 1980, 13 (03) :188-193
[10]  
GODBOLE SP, 1983, THESIS U PITTSBURGH