EXPERIMENTAL-DETERMINATION OF THE QUANTUM-MECHANICAL STATE OF A MOLECULAR VIBRATIONAL-MODE USING FLUORESCENCE TOMOGRAPHY

被引：301

作者：

DUNN, TJ

WALMSLEY, IA

MUKAMEL, S

机构：

[1] UNIV ROCHESTER,INST OPT,ROCHESTER,NY 14627

[2] UNIV ROCHESTER,DEPT CHEM,ROCHESTER,NY 14627

来源：

PHYSICAL REVIEW LETTERS | 1995年 / 74卷 / 06期

关键词：

D O I：

10.1103/PhysRevLett.74.884

中图分类号：

O4 [物理学];

学科分类号：

0702 ;

摘要：

We present a spectroscopic method for the complete characterization of the quantum state of the vibrational mode of a molecule in terms of a phase-space quasiprobability distribution. The distribution for a molecular vibrational mode excited by a short optical pulse is reconstructed from measurements of its time-dependent spectrum of fluorescence. © 1995 The American Physical Society.

引用

页码：884 / 887

页数：4

共 18 条

[1] EXPERIMENTAL-DETERMINATION OF THE H(N = 3) DENSITY-MATRIX FOR 80-KEV H+ ON HE
ASHBURN, JR
CLINE, RA
STONE, CD
VANDERBURGT, PJM
WESTERVELD, WB
RISLEY, JS
[J]. PHYSICAL REVIEW A, 1989, 40 (09): : 4885 - 4901
[2] EXPERIMENTALLY DETERMINED DENSITY-MATRICES FOR H(N=3) FORMED IN H+-HE COLLISIONS FROM 20 TO 100 KEV
ASHBURN, JR
CLINE, RA
VANDERBURGT, PJM
WESTERVELD, WB
RISLEY, JS
[J]. PHYSICAL REVIEW A, 1990, 41 (05): : 2407 - 2421
[3] FEMTOSECOND TIME-RESOLVED MOLECULAR MULTIPHOTON IONIZATION - THE NA2 SYSTEM
BAUMERT, T
GROSSER, M
THALWEISER, R
GERBER, G
[J]. PHYSICAL REVIEW LETTERS, 1991, 67 (27) : 3753 - 3756
[4] A TOMOGRAPHIC APPROACH TO WIGNER FUNCTION
BERTRAND, J
BERTRAND, P
[J]. FOUNDATIONS OF PHYSICS, 1987, 17 (04) : 397 - 405
[5] BERTRAND P, 1985, RECH AEROSPATIALE, V5, P277
[6] DANTUS M, 1987, J CHEM PHYS, V87, P2396
[7] EXPERIMENTAL-DETERMINATION OF THE DYNAMICS OF A MOLECULAR NUCLEAR WAVE-PACKET VIA THE SPECTRA OF SPONTANEOUS EMISSION
DUNN, TJ
SWEETSER, JN
WALMSLEY, IA
RADZEWICZ, C
[J]. PHYSICAL REVIEW LETTERS, 1993, 70 (22) : 3388 - 3391
[8] TIME-DEPENDENT PHYSICAL SPECTRUM OF LIGHT
EBERLY, JH
WODKIEWICZ, K
[J]. JOURNAL OF THE OPTICAL SOCIETY OF AMERICA, 1977, 67 (09) : 1252 - 1261
[9] GERCHBERG RW, 1972, OPTIK, V35, P237
[10] Kemble EC., 1937, FUNDAMENTAL PRINCIPL

← 1 2 →