OFF-RESONANT NONLINEAR OPTICAL-PROPERTIES OF C60 STUDIED BY DEGENERATE 4-WAVE-MIXING

被引：212

作者：

KAFAFI, ZH

LINDLE, JR

PONG, RGS

BARTOLI, FJ

LINGG, LJ

MILLIKEN, J

机构：

[1] Naval Research Laboratory, Washington

来源：

CHEMICAL PHYSICS LETTERS | 1992年 / 188卷 / 5-6期

关键词：

D O I：

10.1016/0009-2614(92)80854-5

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Pure C60 was deposited on optical substrates in vacuo and spectroscopically characterized. A small linear absorption coefficient-alpha = 6 cm-1 was measured at 1.064-mu-m. Time-resolved degenerate four-wave mixing experiments were conducted on films of pure C60 using a 35 ps Nd: YAG laser at 1.064-mu-m. The third-order optical susceptibility chi(xxxx)(3) of C60, derived from its phase conjugate signal. is 7 X 10(-12) esu. The nonlinear optical temporal response was largely laser-pulse limited. Evidence for a fifth-order contribution to the nonlinear optical response was observed at high laser intensities.

引用

页码：492 / 496

页数：5

共 23 条

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