OPTICAL SPECTROSCOPY ON SIZE SELECTED GOLD CLUSTERS DEPOSITED IN RARE-GAS MATRICES

被引:19
作者
HARBICH, W [1 ]
FEDRIGO, S [1 ]
BUTTET, J [1 ]
LINDSAY, DM [1 ]
机构
[1] CUNY CITY COLL,DEPT MED,NEW YORK,NY 10031
来源
ZEITSCHRIFT FUR PHYSIK D-ATOMS MOLECULES AND CLUSTERS | 1991年 / 19卷 / 1-4期
关键词
29.25.Cy; 36.40. +d; 78.40; -q;
D O I
10.1007/BF01448280
中图分类号
O64 [物理化学(理论化学)、化学物理学]; O56 [分子物理学、原子物理学];
学科分类号
070203 ; 070304 ; 081704 ; 1406 ;
摘要
We report on the successful "soft-landing" of size selected Au trimers in solid Krypton matrices. The Au cations are produced by sputtering, mass-selected in a quadrupole mass spectrometer, co-deposited with Krypton on a cooled CaF2 substrate, and neutralized by low energy electrons. The deposition of low kinetic energy cations (10 eV) gives rise to strong excitation bands, detected by the emitted fluorescence light, which are unambiguously attributed to Au trimers. The deposition and fragmentation process is qualitatively discussed.
引用
收藏
页码:157 / 159
页数:3
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