OPTICAL 3RD-HARMONIC GENERATION IN LAYERED PEROVSKITE-TYPE MATERIAL (C10H21NH3)2PBI4

被引：57

作者：

XU, CQ ^{[1
]}

KONDO, T ^{[1
]}

SAKAKURA, H ^{[1
]}

KUMATA, K ^{[1
]}

TAKAHASHI, Y ^{[1
]}

ITO, R ^{[1
]}

机构：

[1] IBM JAPAN LTD,TOKYO RES LAB,TOKYO 102,JAPAN

来源：

SOLID STATE COMMUNICATIONS | 1991年 / 79卷 / 03期

关键词：

D O I：

10.1016/0038-1098(91)90643-A

中图分类号：

O469 [凝聚态物理学];

学科分类号：

070205 ;

摘要：

Optical third-harmonic generation has been investigated over a wide range of wavelengths on a layered perovskite-type material (C10H21NH3)2PbI4, which exhibits prominent two-dimensional exciton effects due to the "natural superlattice" structure. The measured nonlinear optical susceptibility chi(3) (-3-omega; omega, omega, omega) shows large three-photon resonance to the lowest-energy exciton for the fundamental wavelength at 1.53-mu-m. The magnitude of chi(3) reaches 10(-9) esu, which is comparable to the largest reported value on organic materials with one-dimensional conjugated pi-electron structures.

引用

页码：245 / 248

页数：4

共 15 条

[1] CHEMLA DS, 1987, SEMICONDUCT SEMIMET, V24, pCH5
[2] SPECTRUM OF CHI(3)(-3-OMEGA-OMEGA, OMEGA, OMEGA, OMEGA) IN POLYACETYLENE - AN APPLICATION OF THE FREE-ELECTRON LASER IN NONLINEAR OPTICAL SPECTROSCOPY
FANN, WS
BENSON, S
MADEY, JMJ
ETEMAD, S
BAKER, GL
KAJZAR, F
[J]. PHYSICAL REVIEW LETTERS, 1989, 62 (13) : 1492 - 1495
[3] QUANTUM WELLS WITH ENHANCED EXCITON EFFECTS AND OPTICAL NON-LINEARITY
HANAMURA, E
NAGAOSA, N
KUMAGAI, M
TAKAGAHARA, T
[J]. MATERIALS SCIENCE AND ENGINEERING B-SOLID STATE MATERIALS FOR ADVANCED TECHNOLOGY, 1988, 1 (3-4): : 255 - 258
[4] OPTICAL-PROPERTIES DUE TO ELECTRONIC-TRANSITIONS IN 2-DIMENSIONAL SEMICONDUCTORS (CNH2N + 1NH3)2PBI4
ISHIHARA, T
TAKAHASHI, J
GOTO, T
[J]. PHYSICAL REVIEW B, 1990, 42 (17): : 11099 - 11107
[5] EXCITON-STATE IN TWO-DIMENSIONAL PEROVSKITE SEMICONDUCTOR (C10H21NH3)2PBI4
ISHIHARA, T
TAKAHASHI, J
GOTO, T
[J]. SOLID STATE COMMUNICATIONS, 1989, 69 (09) : 933 - 936
[6] RESONANCE ENHANCEMENT IN CUBIC SUSCEPTIBILITY OF LANGMUIR-BLODGETT MULTILAYERS OF POLYDIACETYLENE
KAJZAR, F
MESSIER, J
[J]. THIN SOLID FILMS, 1985, 132 (1-4) : 11 - 19
[7] INTERSPECIMEN COMPARISON OF REFRACTIVE INDEX OF FUSED SILICA
MALITSON, IH
[J]. JOURNAL OF THE OPTICAL SOCIETY OF AMERICA, 1965, 55 (10P1) : 1205 - &
[8] 3RD-ORDER OPTICAL SUSCEPTIBILITY DETERMINATION BY 3RD HARMONIC-GENERATION .1.
MEREDITH, GR
BUCHALTER, B
HANZLIK, C
[J]. JOURNAL OF CHEMICAL PHYSICS, 1983, 78 (03) : 1533 - 1542
[9] Evaluation of Nonlinear Optical Susceptibility of Polydiacetylenes by Third-Harmonic Generation
Nakanishi, H.
Matsuda, H.
Okada, S.
Kato, M.
[J]. POLYMERS FOR ADVANCED TECHNOLOGIES, 1990, 1 (01) : 75 - 79
[10] 3RD-HARMONIC GENERATION IN POLYPHENYLACETYLENE - EXACT DETERMINATION OF NONLINEAR OPTICAL SUSCEPTIBILITIES IN ULTRATHIN FILMS
NEHER, D
WOLF, A
BUBECK, C
WEGNER, G
[J]. CHEMICAL PHYSICS LETTERS, 1989, 163 (2-3) : 116 - 122

← 1 2 →