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STUDIES OF SUPPORTED NICKEL CATALYSTS BY X-RAY PHOTOELECTRON AND ION SCATTERING SPECTROSCOPIES
被引:209
作者
:
WU, M
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV PITTSBURGH,DEPT CHEM,PITTSBURGH,PA 15260
UNIV PITTSBURGH,DEPT CHEM,PITTSBURGH,PA 15260
WU, M
[
1
]
HERCULES, DM
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV PITTSBURGH,DEPT CHEM,PITTSBURGH,PA 15260
UNIV PITTSBURGH,DEPT CHEM,PITTSBURGH,PA 15260
HERCULES, DM
[
1
]
机构
:
[1]
UNIV PITTSBURGH,DEPT CHEM,PITTSBURGH,PA 15260
来源
:
JOURNAL OF PHYSICAL CHEMISTRY
|
1979年
/ 83卷
/ 15期
关键词
:
D O I
:
10.1021/j100478a015
中图分类号
:
O64 [物理化学(理论化学)、化学物理学];
学科分类号
:
070304 ;
081704 ;
摘要
:
Supported nickel catalysts, prepared by impregnation, were studied by two surface sensitive techniques: X-ray photoelectron spectroscopy (ESCA or XPS) and ion scattering spectroscopy (ISS). The nature of the nickel species on the surface was analyzed by ESCA when the support was changed. ESCA-H2 titrations were used to systematically characterize the nickel species as a function of calcination temperature and nickel content. The relationship between the signal intensity ratio of Ni/Al and the bulk nickel content was examined and compared by ESCA and ISS, which have different sampling depths. Nickel shows little interaction with silica but strong interaction with γ-alumina in the impregnated catalysts after calcination. In unreduced silica supported catalysts, the nickel species is NiO. At low nickel content of the unreduced γ-alumina supported catalysts, there are two forms of the nickel present on the surface. At high nickel content, a third species of nickel (NiO) appears after the surface sites of γ-alumina have been filled. The results demonstrate that comparative studies by ESCA and ISS can potentially provide valuable information about the character of surface species on supported catalysts. © 1979 American Chemical Society.
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收藏
页码:2003 / 2008
页数:6
相关论文
共 16 条
[1]
CHEMISTRY OF NICKEL-ALUMINA CATALYSTS
BARTHOLOMEW, CH
论文数:
0
引用数:
0
h-index:
0
机构:
BRIGHAM YOUNG UNIV,DEPT CHEM ENGN SCI,PROVO,UT 84602
BARTHOLOMEW, CH
FARRAUTO, RJ
论文数:
0
引用数:
0
h-index:
0
机构:
BRIGHAM YOUNG UNIV,DEPT CHEM ENGN SCI,PROVO,UT 84602
FARRAUTO, RJ
[J].
JOURNAL OF CATALYSIS,
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X-RAY PHOTOELECTRON-SPECTROSCOPY STUDIES OF RHODIUM ON CHARCOAL CATALYST .2. DISPERSION AS A FUNCTION OF REDUCTION
BRINEN, JS
论文数:
0
引用数:
0
h-index:
0
机构:
AMER CYANAMID CO,CHEM RES DIV,STAMFORD,CT 06904
BRINEN, JS
SCHMITT, JL
论文数:
0
引用数:
0
h-index:
0
机构:
AMER CYANAMID CO,CHEM RES DIV,STAMFORD,CT 06904
SCHMITT, JL
DOUGHMAN, WR
论文数:
0
引用数:
0
h-index:
0
机构:
AMER CYANAMID CO,CHEM RES DIV,STAMFORD,CT 06904
DOUGHMAN, WR
ACHORN, PJ
论文数:
0
引用数:
0
h-index:
0
机构:
AMER CYANAMID CO,CHEM RES DIV,STAMFORD,CT 06904
ACHORN, PJ
SIEGEL, LA
论文数:
0
引用数:
0
h-index:
0
机构:
AMER CYANAMID CO,CHEM RES DIV,STAMFORD,CT 06904
SIEGEL, LA
DELGASS, WN
论文数:
0
引用数:
0
h-index:
0
机构:
AMER CYANAMID CO,CHEM RES DIV,STAMFORD,CT 06904
DELGASS, WN
[J].
JOURNAL OF CATALYSIS,
1975,
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: 295
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EFFECT OF ZINC, GALLIUM, AND GERMANIUM IONS ON STRUCTURAL AND MAGNETIC-PROPERTIES OF NICKEL IONS SUPPORTED ON ALUMINA
CIMINO, A
论文数:
0
引用数:
0
h-index:
0
机构:
CNR,CTR STUDIO STRUTTURA ATTIVITA CATALITICA SISTEM OSSIDI,ROME,ITALY
CIMINO, A
JACONO, ML
论文数:
0
引用数:
0
h-index:
0
机构:
CNR,CTR STUDIO STRUTTURA ATTIVITA CATALITICA SISTEM OSSIDI,ROME,ITALY
JACONO, ML
SCHIAVELLO, M
论文数:
0
引用数:
0
h-index:
0
机构:
CNR,CTR STUDIO STRUTTURA ATTIVITA CATALITICA SISTEM OSSIDI,ROME,ITALY
SCHIAVELLO, M
[J].
JOURNAL OF PHYSICAL CHEMISTRY,
1975,
79
(03)
: 243
-
249
[4]
X-RAY PHOTOELECTRON-SPECTRA OF OXYGEN IN OXIDES OF CO, NI, FE AND ZN
HABER, J
论文数:
0
引用数:
0
h-index:
0
机构:
POLISH ACAD SCI,CATALYSIS & SURFACE CHEM RES LABS,PL-30060 CRACOW,POLAND
POLISH ACAD SCI,CATALYSIS & SURFACE CHEM RES LABS,PL-30060 CRACOW,POLAND
HABER, J
STOCH, J
论文数:
0
引用数:
0
h-index:
0
机构:
POLISH ACAD SCI,CATALYSIS & SURFACE CHEM RES LABS,PL-30060 CRACOW,POLAND
POLISH ACAD SCI,CATALYSIS & SURFACE CHEM RES LABS,PL-30060 CRACOW,POLAND
STOCH, J
UNGIER, L
论文数:
0
引用数:
0
h-index:
0
机构:
POLISH ACAD SCI,CATALYSIS & SURFACE CHEM RES LABS,PL-30060 CRACOW,POLAND
POLISH ACAD SCI,CATALYSIS & SURFACE CHEM RES LABS,PL-30060 CRACOW,POLAND
UNGIER, L
[J].
JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA,
1976,
9
(06)
: 459
-
467
[5]
X-RAY PHOTOELECTRON SPECTROSCOPIC STUDIES OF NICKEL-OXYGEN SURFACES USING OXYGEN AND ARGON ION-BOMBARDMENT
KIM, KS
论文数:
0
引用数:
0
h-index:
0
机构:
PURDUE UNIV,DEPT CHEM,W LAFAYETTE,IN 47906
PURDUE UNIV,DEPT CHEM,W LAFAYETTE,IN 47906
KIM, KS
WINOGRAD, N
论文数:
0
引用数:
0
h-index:
0
机构:
PURDUE UNIV,DEPT CHEM,W LAFAYETTE,IN 47906
PURDUE UNIV,DEPT CHEM,W LAFAYETTE,IN 47906
WINOGRAD, N
[J].
SURFACE SCIENCE,
1974,
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(02)
: 625
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CATALYTIC ALUMINAS - SURFACE MODELS AND CHARACTERIZATION OF SURFACE SITES
KNOZINGER, H
论文数:
0
引用数:
0
h-index:
0
机构:
Institut fur Physikalische Chernie, Universiat Munchen, Sophiezstrasse 11, 3000
KNOZINGER, H
RATNASAMY, P
论文数:
0
引用数:
0
h-index:
0
机构:
Institut fur Physikalische Chernie, Universiat Munchen, Sophiezstrasse 11, 3000
RATNASAMY, P
[J].
CATALYSIS REVIEWS-SCIENCE AND ENGINEERING,
1978,
17
(01):
: 31
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70
[7]
LOJACONO M, 1971, J PHYS CHEM-US, V75, P1044, DOI 10.1021/j100678a005
[8]
STUDIES OF NICKEL-TUNGSTEN-ALUMINA CATALYSTS BY X-RAY PHOTOELECTRON-SPECTROSCOPY
NG, KT
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
NG, KT
HERCULES, DM
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
HERCULES, DM
[J].
JOURNAL OF PHYSICAL CHEMISTRY,
1976,
80
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EFFECT OF NEXT NEAREST NEIGHBOR ION ON X-RAY PHOTOELECTRON-SPECTRA OF 2P LEVELS FOR CO-2+, NI-2+ AND CU-2+ IN MGO
OKU, M
论文数:
0
引用数:
0
h-index:
0
机构:
TOHOKU UNIV, IRON STEEL & OTHER MET RES INST, SENDAI, MIYAGI 980, JAPAN
TOHOKU UNIV, IRON STEEL & OTHER MET RES INST, SENDAI, MIYAGI 980, JAPAN
OKU, M
HIROKAWA, K
论文数:
0
引用数:
0
h-index:
0
机构:
TOHOKU UNIV, IRON STEEL & OTHER MET RES INST, SENDAI, MIYAGI 980, JAPAN
TOHOKU UNIV, IRON STEEL & OTHER MET RES INST, SENDAI, MIYAGI 980, JAPAN
HIROKAWA, K
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JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA,
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SURFACE STUDY OF COBALT-MOLYBDENA-ALUMINA CATALYSTS USING X-RAY PHOTOELECTRON-SPECTROSCOPY
PATTERSON, TA
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
PATTERSON, TA
CARVER, JC
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
CARVER, JC
LEYDEN, DE
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
LEYDEN, DE
HERCULES, DM
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
HERCULES, DM
[J].
JOURNAL OF PHYSICAL CHEMISTRY,
1976,
80
(15)
: 1700
-
1708
←
1
2
→
共 16 条
[1]
CHEMISTRY OF NICKEL-ALUMINA CATALYSTS
BARTHOLOMEW, CH
论文数:
0
引用数:
0
h-index:
0
机构:
BRIGHAM YOUNG UNIV,DEPT CHEM ENGN SCI,PROVO,UT 84602
BARTHOLOMEW, CH
FARRAUTO, RJ
论文数:
0
引用数:
0
h-index:
0
机构:
BRIGHAM YOUNG UNIV,DEPT CHEM ENGN SCI,PROVO,UT 84602
FARRAUTO, RJ
[J].
JOURNAL OF CATALYSIS,
1976,
45
(01)
: 41
-
53
[2]
X-RAY PHOTOELECTRON-SPECTROSCOPY STUDIES OF RHODIUM ON CHARCOAL CATALYST .2. DISPERSION AS A FUNCTION OF REDUCTION
BRINEN, JS
论文数:
0
引用数:
0
h-index:
0
机构:
AMER CYANAMID CO,CHEM RES DIV,STAMFORD,CT 06904
BRINEN, JS
SCHMITT, JL
论文数:
0
引用数:
0
h-index:
0
机构:
AMER CYANAMID CO,CHEM RES DIV,STAMFORD,CT 06904
SCHMITT, JL
DOUGHMAN, WR
论文数:
0
引用数:
0
h-index:
0
机构:
AMER CYANAMID CO,CHEM RES DIV,STAMFORD,CT 06904
DOUGHMAN, WR
ACHORN, PJ
论文数:
0
引用数:
0
h-index:
0
机构:
AMER CYANAMID CO,CHEM RES DIV,STAMFORD,CT 06904
ACHORN, PJ
SIEGEL, LA
论文数:
0
引用数:
0
h-index:
0
机构:
AMER CYANAMID CO,CHEM RES DIV,STAMFORD,CT 06904
SIEGEL, LA
DELGASS, WN
论文数:
0
引用数:
0
h-index:
0
机构:
AMER CYANAMID CO,CHEM RES DIV,STAMFORD,CT 06904
DELGASS, WN
[J].
JOURNAL OF CATALYSIS,
1975,
40
(03)
: 295
-
300
[3]
EFFECT OF ZINC, GALLIUM, AND GERMANIUM IONS ON STRUCTURAL AND MAGNETIC-PROPERTIES OF NICKEL IONS SUPPORTED ON ALUMINA
CIMINO, A
论文数:
0
引用数:
0
h-index:
0
机构:
CNR,CTR STUDIO STRUTTURA ATTIVITA CATALITICA SISTEM OSSIDI,ROME,ITALY
CIMINO, A
JACONO, ML
论文数:
0
引用数:
0
h-index:
0
机构:
CNR,CTR STUDIO STRUTTURA ATTIVITA CATALITICA SISTEM OSSIDI,ROME,ITALY
JACONO, ML
SCHIAVELLO, M
论文数:
0
引用数:
0
h-index:
0
机构:
CNR,CTR STUDIO STRUTTURA ATTIVITA CATALITICA SISTEM OSSIDI,ROME,ITALY
SCHIAVELLO, M
[J].
JOURNAL OF PHYSICAL CHEMISTRY,
1975,
79
(03)
: 243
-
249
[4]
X-RAY PHOTOELECTRON-SPECTRA OF OXYGEN IN OXIDES OF CO, NI, FE AND ZN
HABER, J
论文数:
0
引用数:
0
h-index:
0
机构:
POLISH ACAD SCI,CATALYSIS & SURFACE CHEM RES LABS,PL-30060 CRACOW,POLAND
POLISH ACAD SCI,CATALYSIS & SURFACE CHEM RES LABS,PL-30060 CRACOW,POLAND
HABER, J
STOCH, J
论文数:
0
引用数:
0
h-index:
0
机构:
POLISH ACAD SCI,CATALYSIS & SURFACE CHEM RES LABS,PL-30060 CRACOW,POLAND
POLISH ACAD SCI,CATALYSIS & SURFACE CHEM RES LABS,PL-30060 CRACOW,POLAND
STOCH, J
UNGIER, L
论文数:
0
引用数:
0
h-index:
0
机构:
POLISH ACAD SCI,CATALYSIS & SURFACE CHEM RES LABS,PL-30060 CRACOW,POLAND
POLISH ACAD SCI,CATALYSIS & SURFACE CHEM RES LABS,PL-30060 CRACOW,POLAND
UNGIER, L
[J].
JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA,
1976,
9
(06)
: 459
-
467
[5]
X-RAY PHOTOELECTRON SPECTROSCOPIC STUDIES OF NICKEL-OXYGEN SURFACES USING OXYGEN AND ARGON ION-BOMBARDMENT
KIM, KS
论文数:
0
引用数:
0
h-index:
0
机构:
PURDUE UNIV,DEPT CHEM,W LAFAYETTE,IN 47906
PURDUE UNIV,DEPT CHEM,W LAFAYETTE,IN 47906
KIM, KS
WINOGRAD, N
论文数:
0
引用数:
0
h-index:
0
机构:
PURDUE UNIV,DEPT CHEM,W LAFAYETTE,IN 47906
PURDUE UNIV,DEPT CHEM,W LAFAYETTE,IN 47906
WINOGRAD, N
[J].
SURFACE SCIENCE,
1974,
43
(02)
: 625
-
643
[6]
CATALYTIC ALUMINAS - SURFACE MODELS AND CHARACTERIZATION OF SURFACE SITES
KNOZINGER, H
论文数:
0
引用数:
0
h-index:
0
机构:
Institut fur Physikalische Chernie, Universiat Munchen, Sophiezstrasse 11, 3000
KNOZINGER, H
RATNASAMY, P
论文数:
0
引用数:
0
h-index:
0
机构:
Institut fur Physikalische Chernie, Universiat Munchen, Sophiezstrasse 11, 3000
RATNASAMY, P
[J].
CATALYSIS REVIEWS-SCIENCE AND ENGINEERING,
1978,
17
(01):
: 31
-
70
[7]
LOJACONO M, 1971, J PHYS CHEM-US, V75, P1044, DOI 10.1021/j100678a005
[8]
STUDIES OF NICKEL-TUNGSTEN-ALUMINA CATALYSTS BY X-RAY PHOTOELECTRON-SPECTROSCOPY
NG, KT
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
NG, KT
HERCULES, DM
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
HERCULES, DM
[J].
JOURNAL OF PHYSICAL CHEMISTRY,
1976,
80
(19)
: 2094
-
2102
[9]
EFFECT OF NEXT NEAREST NEIGHBOR ION ON X-RAY PHOTOELECTRON-SPECTRA OF 2P LEVELS FOR CO-2+, NI-2+ AND CU-2+ IN MGO
OKU, M
论文数:
0
引用数:
0
h-index:
0
机构:
TOHOKU UNIV, IRON STEEL & OTHER MET RES INST, SENDAI, MIYAGI 980, JAPAN
TOHOKU UNIV, IRON STEEL & OTHER MET RES INST, SENDAI, MIYAGI 980, JAPAN
OKU, M
HIROKAWA, K
论文数:
0
引用数:
0
h-index:
0
机构:
TOHOKU UNIV, IRON STEEL & OTHER MET RES INST, SENDAI, MIYAGI 980, JAPAN
TOHOKU UNIV, IRON STEEL & OTHER MET RES INST, SENDAI, MIYAGI 980, JAPAN
HIROKAWA, K
[J].
JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA,
1977,
10
(02)
: 103
-
110
[10]
SURFACE STUDY OF COBALT-MOLYBDENA-ALUMINA CATALYSTS USING X-RAY PHOTOELECTRON-SPECTROSCOPY
PATTERSON, TA
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
PATTERSON, TA
CARVER, JC
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
CARVER, JC
LEYDEN, DE
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
LEYDEN, DE
HERCULES, DM
论文数:
0
引用数:
0
h-index:
0
机构:
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
UNIV GEORGIA,DEPT CHEM,ATHENS,GA 30602
HERCULES, DM
[J].
JOURNAL OF PHYSICAL CHEMISTRY,
1976,
80
(15)
: 1700
-
1708
←
1
2
→