THE INTRINSIC LINE-WIDTH OF THE PLASMON RESONANCES IN METAL MICROCLUSTERS AT VERY LOW-TEMPERATURES - QUANTAL SURFACE FLUCTUATIONS

被引:31
作者
PACHECO, JM
BROGLIA, RA
MOTTELSON, BR
机构
[1] UNIV MILAN,DIPARTMENTO FIS,I-20133 MILAN,ITALY
[2] NORDITA,DK-2100 COPENHAGEN,DENMARK
[3] IST NAZL FIS NUCL,I-20133 MILAN,ITALY
来源
ZEITSCHRIFT FUR PHYSIK D-ATOMS MOLECULES AND CLUSTERS | 1991年 / 21卷 / 03期
关键词
D O I
10.1007/BF01426388
中图分类号
O64 [物理化学(理论化学)、化学物理学]; O56 [分子物理学、原子物理学];
学科分类号
070203 ; 070304 ; 081704 ; 1406 ;
摘要
The line shape of the plasmon resonance in a cold, small sodium cluster (Na8) is calculated taking into account its coupling to the quantal quadrupole fluctuations of the cluster shape. This coupling is found to give rise to a small damping factor (GAMMA/h-omega-1 approximately 0.03, where h-omega-1 denotes the energy centroid and GAMMA the full width at half maximum of the resonance), and to an asymmetric line shape with Gaussian behaviour in the wings.
引用
收藏
页码:289 / 292
页数:4
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